科研成果

2022
Li Y, Zhang RQ, He S, Chiaradia M, Li XH. Pulsed exsolution of magmatic ore-forming fluids in tin-tungsten systems: a SIMS cassiterite oxygen isotope record. Mineralium Deposita. 2022;57:343-352.Abstract
Y Utilizing in situ oxygen isotope analysis, we demonstrate the potential of cassiterite as a robust recorder of fluid source and evolution. Cassiterite is an ore mineral, and its mineral-water oxygen isotope fractionation factor is only weakly temperature-dependent. Unlike most explored gangue minerals such as quartz, cassiterite can provide a direct and robust archive of ore-forming fluids, e.g., fluid oxygen isotope composition (delta O-18 values). Core and rim domains of a representative cassiterite crystal from the Piaotang tin-tungsten (Sn-W) deposit, China, are characterized by contrasting delta O-18 values. Cassiterite delta O-18 values are -2.14 +/- 0.41 parts per thousand for the core and 2.36 +/- 0.36 parts per thousand for the rim, which equate to fluid delta O-18 values of similar to 4.1 parts per thousand (core) and similar to 8.6 parts per thousand (rim). Additionally, the cassiterite rim is enriched in niobium (Nb) and tantalum (Ta) compared to the mineral core. The delta O-18, and Nb and Ta data are interpreted to reflect core to rim crystallization from distinct pulses of magmatic-hydrothermal fluids that possessed a discrete oxygen isotopic, and Nb and Ta composition. Such a pulsed process could be a common feature for Sn-W deposits, and is critical to the formation of giant deposits with high metal grades. Involvement of meteoric water associated with the first mineralization stage reaches similar to 33%, but is limited (similar to 7%) in the second (main) mineralization stage. Therefore, cooling induced by fluid mixing may not be necessary for tin deposition, and our new findings invite a reassessment of the role of meteoric water in other Sn-W deposits. Our petrologic modelling shows that fluids exsolved from a 10 - 15 km(3) parental granitic magma can yield the Sn-W endowments recorded at Piaotang. Further, during magma fractionation, Sn and W are preferentially transferred into fluids compared to Nb and Ta. As a consequence, fluid chemistry is the primary factor controlling metal endowment and zoning in W-Sn deposits, as observed at Piaotang, and explains the predominant magmatic origin of Nb-Ta deposits.
Qi Liu, Xun Pang, James Vreeland, “The Effect of China's Cross-Currency Swap Agreements on Foreign Policy Preferences," Working Paper. 2022.Abstract
How does China’s growing financial power reshape the structure of world politics? Does the expansion of China’s global influence come at the expense of the United States? A growing body of research in International Relations (IR) finds that China is increasingly using its economic power to gain leverage in international politics and engage countries to support its foreign policy. This paper addresses the question of whether “the rise of the Renminbi" – China’s entry into global monetary affairs through its BSA network – boosts its political influence and diminishes US political power on the global stage. To tackle the identification problem, we employ a Bayesian causal inference method devel-oped by Pang et al. (2021): bpCausal. Our analysis reveals intriguing results. First, we find that on average China’s BSAs have statistically a significant short-run causal effect of on governments’ expressed preferences over global issues. That is, BSAs bring the foreign policy ideal points of China and its partner states closer together in the year after a BSA is signed. Interestingly, while BSAs shift signatories closer to China’s ideal point in the UNGA, we find no evidence that BSAs pull countries away from the positions of the United States. On the contrary, weak evidence suggests that governments are moving closer to the United States in the median run, holding all other things constant, though the impact is much smaller compared to moving closer toChina.
Xuefei Ma, Zhaofeng Tan KLYZ. Quantitative study on the interference of OH radicalmeasurement in the air pollution complex. Chinese Science Bulletin [Internet]. 2022;67:3724-3736. 访问链接
Han J, Liu C, Zhang Y, Guan Y, Zhang X, Yu W, Tang Z, Liang Y, Wu C, Zheng S, et al. Quasi-2D Ruddlesden-Popper Perovskites with Low Trap-States for High Performance Flexible Self-Powered Ultraviolet Photodetectors. ADVANCED OPTICAL MATERIALS. 2022;10.
Yang X, Lu K, Ma X, Gao Y, Tan Z, Wang H, Chen X, Li X, HUANG X, He L, et al. Radical chemistry in the Pearl River Delta: observations and modeling of OH and HO2 radicals in Shenzhen 2018. 2022.
Dang C, Wang J, He Y, Yang S, Chen Y, Liu T, Fu J, Chen Q, Ni J. Rare biosphere regulates the planktonic and sedimentary bacteria by disparate ecological processes in a large source water reservoir. Water ResearchWater Research. 2022;216.Abstract
The bacteria in the water column and surface sediments are inherently intertwined and inseparable in aquatic ecosystems, yet little is known about the integrated spatiotemporal dynamics and driving mechanisms of both planktonic and sedimentary bacterial communities in reservoirs. By investigating the planktonic and sedimentary bacteria during four seasons from 88 samples of 11 representative sites across the Danjiangkou reservoir, we depicted an integrated biogeographic pattern of bacterial communities in the water source of the world's largest water diversion project. Our study revealed both planktonic (mantel r = 0.502, P = 0.001) and sedimentary (mantel r = 0.131, P = 0.009) bacterial communities were significantly correlated with environmental heterogeneity, but a weak disparity along spatial heterogeneity, and the significant seasonal dynamics of planktonic (mantel r = 0.499, P = 0.001) rather than sedimentary bacteria. Particularly, rare biosphere played a main role in determining the community succession in the reservoir. It not only exhibited a more striking environmental separation than abundant taxa but also was an essential part in mediating spatiotemporal shifts of planktonic bacteria and maintaining the stability of bacterial community. These rare bacteria were respectively mediated by stochastic (62.68%) and selective (79.60%) processes in water and sediments despite abundant taxa being largely determined by stochastic processes (86.88-93.96%). Overall, our study not only fills a gap in understanding the bacterial community dynamics and underlying drivers in source water reservoirs, but also highlights the particular importance of rare bacteria in mediating biogeochemical cycles in world's large reservoir ecosystems.
Iyer G, Ou Y, Edmonds J, Fawcett AA, Hultman N, McFarland J, Fuhrman J, Waldhoff S, McJeon H. Ratcheting of climate pledges needed to limit peak global warming. Nature Climate Change. 2022;12(12):1129-1135.
Deng H, Poonoosamy J, Molins S. A reactive transport modeling perspective on the dynamics of interface-coupled dissolution-precipitation. Applied geochemistry. 2022;137:105207.
Zhang C, Yang H, Zhao Y, Ma L, Larson ED, Greig C. Realizing ambitions: A framework for iteratively assessing and communicating national decarbonization progress. iScience [Internet]. 2022;25:103695. 访问链接Abstract
Summary A growing number of governments are pledging to achieve net-zero greenhouse gas emissions by mid-century. Despite such ambitions, realized emissions reductions continue to fall alarmingly short of modeled energy transition pathways for achieving net-zero. This gap is largely a result of the difficulty of realistically modeling all the techno-economic and sociopolitical capabilities that are required to deliver actual emissions reductions. This limitation of models suggests the need for an energy-systems analytical framework that goes well beyond energy-system modeling in order to close the gap between ambition and reality. Toward that end, we propose the Emissions-Sustainability-Governance-Operation (ESGO) framework for structured assessment and transparent communication of national capabilities and realization. We illustrate the critical role of energy modeling in ESGO using recent net-zero modeling studies for the world's two largest emitters, China and the United States. This illustration leads to recommendations for improvements to energy-system modeling to enable more productive ESGO implementation.
Zhang Z, Zhang Y, Guo X, Wang D, Lao Y, Qu B, Xiao L, Chen Z. Realizing High-Efficiency and Stable Perovskite Solar Cells via Double-Perovskite Nanocrystal Passivation. ACS APPLIED ENERGY MATERIALS. 2022;5:1169-1174.
Liu YJ, Mo J. Real-Time Monitoring of Indoor Organic Compounds. In: Zhang Y, Hopke PK, Mandin C Handbook of Indoor Air Quality. Singapore: Springer Nature; 2022. pp. 1–24.
Jeong D, Seco R, Emmons L, Schwantes R, Liu YJ, McKinney KA, Martin ST, Keutsch FN, Gu D, Guenther AB, et al. Reconciling Observed and Predicted Tropical Rainforest OH Concentrations. Journal of Geophysical Research: Atmospheres [Internet]. 2022;127:e2020JD032901. 访问链接Abstract
Abstract We present OH observations made in Amazonas, Brazil during the Green Ocean Amazon campaign (GoAmazon2014/5) from February to March of 2014. The average diurnal variation of OH peaked with a midday (10:00?15:00) average of 1.0 ? 106 (±0.6 ? 106) molecules cm?3. This was substantially lower than previously reported in other tropical forest photochemical environments (2?5 ? 106 molecules cm?3) while the simulated OH reactivity was lower. The observational data set was used to constrain a box model to examine how well current photochemical reaction mechanisms can simulate observed OH. We used one near-explicit mechanism (MCM v3.3.1) and four condensed mechanisms (i.e., RACM2, MOZART-T1, CB05, CB6r2) to simulate OH. A total of 14 days of analysis shows that all five chemical mechanisms were able to explain the measured OH within instrumental uncertainty of 40% during the campaign in the Amazonian rainforest environment. Future studies are required using more reliable NOx and VOC measurements to further investigate discrepancies in our understanding of the radical chemistry in the tropical rainforest.
Zhao J, Xiong R*, Xie J, Shi B, Yu Z, Gao W, Huang T. Reconstructing Clear Image for High-Speed Motion Scene with a Retina-Inspired Spike Camera. IEEE Transactions on Computational Imaging [Internet]. 2022;8:12-27. PDFAbstract
Conventional digital cameras typically accumulate all the photons within an exposure period to form a snapshot image. It requires the scene to be quite still during the imaging time, otherwise it would result in blurry image for the moving objects. Recently, a retina-inspired spike camera has been proposed and shown great potential for recording high-speed motion scenes. Instead of capturing the visual scene by a single snapshot, the spike camera records the dynamic light intensity variation continuously. Each pixel on spike camera sensor accumulates the incoming photons independently and persistently, which fires a spike and restarts the photon accumulation immediately once the dispatch threshold is reached, producing a continuous stream of spikes recorded at very high temporal resolution. To recover the dynamic scene from captured spike stream, this paper presents an image reconstruction approach for spike camera. In order to generate high-quality reconstruction, we investigate the temporal correlation along motion trajectories and exploit it via adaptive temporal filtering. In particular, we present a hierarchical motion-aligned temporal filtering scheme, combining short-term filtering with long-term filtering to take advantage of long-term temporal correlation with low model complexity. Experimental results demonstrate that the proposed scheme outperforms the existing schemes significantly, producing much better objective and subjective qualities for spike camera image reconstruction.
Fu T, Zeng M, Liu S, Liu H, HUANG R, Wu Y. Record-high 2P r= 60 $μ$C/cm 2 by Sub-5ns Switching Pulse in Ferroelectric Lanthanum-doped HfO 2 with Large Single Grain of Orthorhombic Phase> 38 nm, in 2022 International Electron Devices Meeting (IEDM). IEEE; 2022:6–5.
Clarens AF, Fauvel C, Fuhrman J, Ou Y, McJeon HC, Shobe W, Doney S. Regional Implications of Carbon Dioxide Removal on Achieving Net-Zero Emissions Targets. AGU Fall Meeting Abstracts. 2022;2022:GC26F-05.
Ma Y, Wu Z, Lu CQ. The relationship between job insecurity and employee information security behavior: An exploratory study, in The 2022 Academic Annual Meeting of the Managerial Psychology Professional Committee of the Chinese Association of Social Psychology (The 4th China Managerial Psychology/Organizational Behavior Forum). Kunming, China; 2022.
Bu Y, Li H, Wei C, Liu M, Li J. On the relationship between supervisor-supervisee gender difference and scientific impact of doctoral dissertations: Evidence from Humanities and Social Sciences in China. Journal of Information Science. 2022;48(4):492-502.
Liu N, Hu H, Ma W, Deng Y, Dimitrov D, Wang Q, Shrestha N, Su X, Feng K, Liu Y, et al. Relationships Between Soil Microbial Diversities Across an Aridity Gradient in Temperate Grasslands. Microbial Ecology. 2022;85:1013-1027.Abstract
Soil microbes assemble in highly complex and diverse microbial communities, and microbial diversity patterns and their drivers have been studied extensively. However, diversity correlations and co-occurrence patterns between bacterial, fungal, and archaeal domains and between microbial functional groups in arid regions remain poorly understood. Here we assessed the relationships between the diversity and abundance of bacteria, fungi, and archaea and explored how environmental factors influence these relationships. We sampled soil along a 1500-km-long aridity gradient in temperate grasslands of Inner Mongolia (China) and sequenced the 16S rRNA gene of bacteria and archaea and the ITS2 gene of fungi. The diversity correlations and co-occurrence patterns between bacterial, fungal, and archaeal domains and between different microbial functional groups were evaluated using α-diversity and co-occurrence networks based on microbial abundance. Our results indicate insignificant correlations among the diversity patterns of bacterial, fungal, and archaeal domains using α-diversity but mostly positive correlations among diversity patterns of microbial functional groups based on α-diversity and co-occurrence networks along the aridity gradient. These results suggest that studying microbial diversity patterns from the perspective of functional groups and co-occurrence networks can provide additional insights on patterns that cannot be accessed using only overall microbial α-diversity. Increase in aridity weakens the diversity correlations between bacteria and fungi and between bacterial and archaeal functional groups, but strengthens the positive diversity correlations between bacterial functional groups and between fungal functional groups and the negative diversity correlations between bacterial and fungal functional groups. These variations of the diversity correlations are associated with the different responses of microbes to environmental factors, especially aridity. Our findings demonstrate the complex responses of microbial community structure to environmental conditions (especially aridity) and suggest that understanding diversity correlations and co-occurrence patterns between soil microbial groups is essential for predicting changes in microbial communities under future climate change in arid regions.
Zu K, Wang Z. Research progress on the elevational distribution of mountain species in response to climate change. Biodiversity ScienceBiodiversity Science. 2022;30:21451.
Zhang T, Li D, Lu X. Response of runoff components to climate change in the source-region of the Yellow River on the Tibetan plateau. Hydrological Processes [Internet]. 2022;36(6):e14633. 访问链接Abstract
Abstract Climate change will likely increase the total streamflow in most headwaters on the Tibetan Plateau in the next decades, yet the response of runoff components to climate change and permafrost thaw remain largely uncertain. Here, we investigate the changes in runoff components under a changing climate, based on a high-resolution cryosphere-hydrology model (Spatial Processes in Hydrology model, SPHY) and multi-decadal streamflow observations at the upstream (Jimai) and downstream stations (Maqu and Tangnaihai) in the source-region of the Yellow River (SYR). We find that rainfall flow dominates the runoff regime in SYR (contributions of 48%?56%), followed by snowmelt flow (contributions of 26%/23% at Maqu/Tangnaihai). Baseflow is more important at Jimai (32%) than at the the downstream stations (21%?23%). Glacier meltwater from the Anyê Maqên and Bayankala Mountains contributes negligibly to the downstream total runoff. With increasing temperature and precipitation, the increase in total runoff is smaller in the warm and wet downstream stations than in the cold and dry upstream station. This is because of a higher increase in evapotranspiration and a larger reduction in snowmelt flow in the downstream region in response to a warming climate. With temperature increase, there is less increase in rainfall flow in the downstream region due to increased water loss through evapotranspiration. Meanwhile, the decline in snowmelt flow is larger further downstream, which can negatively impact the spring irrigation for the whole Yellow River basin that supports the livelihoods of 140 million people. Importantly, we find that baseflow plays an increasingly important role in the permafrost-dominated upstream region with atmospheric warming and permafrost thaw, accompanied by decreased surface flow. These findings improve our current understanding of how different hydrological processes respond to climate change and provide insights for optimizing hydropower and irrigation systems in the entire Yellow River basin under a rapidly changing climate.

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