科研成果

2021
Xu N, Wang TT, Li X, Tang RZ, Guo S, Hu M. Chemical Characteristics and Source Apportionment of Organic Aerosols in Atmospheric PM2.5 in Winter in Beijing. Huanjing Kexue/Environmental ScienceHuanjing Kexue/Environmental ScienceHuanjing Kexue/Environmental Science. 2021;42:2101-2109.Abstract
To explore the concentrations, characteristics, and sources of organic aerosols in winter in Beijing, atmospheric fine particulate matter (PM2.5) samples were collected from November 10, 2016 to December 10, 2016. One hundred and twenty-nine particulate organic matters (POM) were quantified by gas chromatography-mass spectrometry, accounting for approximately 9.3%±1.2% of the total concentration of organic matter. The most abundant class was sugar, among which levoglucosan alone accounted for 18% of the quantified organic matter mass. The next most abundant classes were alkanoic acids, normal alkanes, dicarboxylic acids, and polycyclic aromatic hydrocarbons. The influence of winter heating and biomass burning emissions on organic aerosols in winter in Beijing was analyzed by the characteristics of the molecular markers in the POM. Compared with those during the non-heating period, the concentrations and proportions of hopane species, which are tracers for fossil fuels, increased in the organic matters during the heating period. Moreover, the influence of coal burning emissions on the distribution of hopane species was enhanced. The species with the maximum concentration and carbon predominance index in n-alkanes also reflected the influence of enhanced fossil fuel emissions. The results of the concentration-weighted trajectory model for levoglucosan, a tracer for biomass combustion, suggested that straw burning pollution in the surrounding areas of Beijing would affect the composition of organic aerosols in Beijing via airmass transport. A molecular marker-based chemical mass balance model was used to apportion the sources of organic carbon in the winter of 2016 in Beijing, and the results were compared with those of research in 2006 to quantify the changes in the source contributions over 10 years. The contribution of motor vehicles increased significantly in 2016 compared with that in 2006, whereas the contribution of coal burning and wood burning decreased to a large extent. The contribution of cooking emissions could not be ignored. Therefore, the control of motor vehicle and cooking emissions is of great importance to reduce the problem of PM2.5 pollution in winter in Beijing. © 2021, Science Press. All right reserved.
Chen X, Ren Z-Y, Li D-L, Liu T, Wang K, Shen Z-Q, Ellingsen SP, Sobolev AM, Mei Y, Li J-J, et al. Chemically Fresh Gas Inflows Detected in a Nearby High-mass Star-forming Region. \apjl. 2021;923:L20.
Li S, Cao S, Duan X, Zhang Y, Gong J, Xu X, Guo Q, Meng X, Bertrand M, Zhang JJ. Children's lung function in relation to changes in socioeconomic, nutritional, and household factors over 20 years in Lanzhou. Journal of Thoracic DiseaseJournal of Thoracic Disease. 2021;13:4574-4588.
Song X, Liu C, Zhang Y. Chinese College Students’ Source Selection and Use in Searching for Health and Wellness Information Online. Information Processing and Management [Internet]. 2021;58(3):102489. 访问链接
Zheng Y, Mou N, Zhang L, Makkonen T, Yang T. Chinese tourists in Nordic countries: An analysis of spatio-temporal behavior using geo-located travel blog data. Computers Environment and Urban Systems. 2021;85:101561.
Min C, Chen Q, Yan E, Bu Y, Sun J. Citation cascade and the evolution of topic relevance. Journal of the Association for Information Science and Technology. 2021;72(1):110-127.
Xue T, Zhu T, Peng W, Guan T, Zhang S, Zheng Y, Geng G, Zhang Q. Clean Air Actions in China, PM2.5 Exposure, and Household Medical Expenditures: a Quasi-Experimental Study [J]. PLOS Medicine. PLoS Medicine. 2021;18(1):1003480.
Janeway MG, Zhao X, Rosenthaler M, Zuo Y, Balasubramaniyan K, Poulson M, Neufeld M, Siracuse JJ, Takahashi CE, Allee L, et al. Clinical Diagnostic Phenotypes in Hospitalizations Due to Self-Inflicted Firearm Injury. Journal of Affective Disorders. 2021;278:172–180.Abstract
Hospitalized self-inflicted firearm injuries have not been extensively studied, particularly regarding clinical diagnoses at the index admission. The objective of this study was to discover the diagnostic phenotypes (DPs) or clusters of hospitalized self-inflicted firearm injuries. Using Nationwide Inpatient Sample data in the US from 1993 to 2014, we used International Classification of Diseases, Ninth Revision codes to identify self-inflicted firearm injuries among those ≥18 years of age. The 25 most frequent diagnostic codes were used to compute a dissimilarity matrix and the optimal number of clusters. We used hierarchical clustering to identify the main DPs. The overall cohort included 14072 hospitalizations, with self-inflicted firearm injuries occurring mainly in those between 16 to 45 years of age, black, with co-occurring tobacco and alcohol use, and mental illness. Out of the three identified DPs, DP1 was the largest (n=10,110), and included most common diagnoses similar to overall cohort, including major depressive disorders (27.7%), hypertension (16.8%), acute post hemorrhagic anemia (16.7%), tobacco (15.7%) and alcohol use (12.6%). DP2 (n=3,725) was not characterized by any of the top 25 ICD-9 diagnoses codes, and included children and peripartum women. DP3, the smallest phenotype (n=237), had high prevalence of depression similar to DP1, and defined by fewer fatal injuries of chest and abdomen. There were three distinct diagnostic phenotypes in hospitalizations due to self-inflicted firearm injuries. Further research is needed to determine how DPs can be used to tailor clinical care and prevention efforts.
Fu P, Schoenball M, Ajo-Franklin JB, Chai C, Maceira M, Morris JP, Wu H, Knox H, Schwering PC, White MD, et al. Close observation of hydraulic fracturing at EGS Collab Experiment 1: Fracture trajectory, microseismic interpretations, and the role of natural fractures. Journal of Geophysical Research: Solid Earth [Internet]. 2021;126:e2020JB020840. 访问链接
Zhang S, Wu Y, Liu X, Qian J, CHEN J, Han L, Dai* H. Co-benefits of deep carbon reduction on air quality and health improvement in Sichuan Province of China. Environmental Research Letters [Internet]. 2021. 访问链接
Wang J, Chen J, Yang X, Liu L, Wu C, Lu L, Li L, Wu Y*. Common brain substrates underlying auditory speech priming and perceived spatial separation. Frontiers in Neuroscience. 2021;15:158.
Fonseca EU, Yang W, Wang X, Rossi R, Logan BE. Comparison of different chemical treatments of brush and flat carbon electrodes to improve performance of microbial fuel cells. Bioresource technology. 2021;342:125932.
Fonseca EU, Yang W, Wang X, Rossi R, Logan BE. Comparison of different chemical treatments of brush and flat carbon electrodes to improve performance of microbial fuel cells. Bioresource technology. 2021;342:125932.
Zhou Y, Lu X, Yu B, Wang D, Zhao C, Yang Q, Zhang Q, Tan Y, Wang X, Guo J. Comparison of neonicotinoid residues in soils of different land use types. Science of the Total Environment [Internet]. 2021;782. 访问链接Abstract
Neonicotinoid insecticides (NEOs) have attracted particular attention in recent years due to their wide occurrence and potential impacts on the ecosystem and human health. This study aimed to compare the composition and level of NEOs in soils of different land use types. Two rounds of sampling were performed in Tianjin, China, with 158 soil samples in fall and 61 soil samples in spring collected from five types of land, i.e., greenhouse, orchard, farm, park and residential area. The concentrations of eight NEOs, i.e., imidacloprid (IMI), acetamiprid (ACE), thiamethoxam (THX), clothianidin (CLO), thiacloprid (THA), dinotefuran (DIN), nitenpyram (NIT) and flonicamid (FLO), were analyzed in the soil samples using LC-MS/MS. Six NEOs were detected, with IMI, ACE and THX being the most frequently detected ones. Concentrations of NEOs (arithmetic means in fall and spring, respectively) in greenhouse were the highest (2.52×102 and 4.59×102 ng g−1), followed by in orchard (35.1 and 1.31×102 ng g−1), park (50.4 and 1.02×102 ng g−1), residential area (20.2 and 1.38×102 ng g−1) and farm (25.5 and 84.2 ng g−1). The contribution of individual NEO varied in soils of different land use types. Both IMI and THX were largely used in greenhouse, while IMI was the main NEO in the other four lands. The NEO levels in soils planted with different crops varied greatly. Extremely high levels of NEOs (>103 ng g−1) were observed in soils planted with watermelon, tomato and peach in greenhouse. The ubiquitous presence of NEOs in soils deserves more attention, particularly in greenhouse. © 2021 Elsevier B.V.
Comparison study on atomic and molecular ellipticity dependence ofhigh-order harmonic generation. PHYSICAL REVIEW A [Internet]. 2021;103(4):043115. 访问链接Abstract
We systematically investigate ellipticity dependence of high-order harmonic generation of Ar and N2 in intense elliptically polarized laser fields. The experimental normalized ratios of low-order harmonic intensity to high-order harmonic intensity increase with ellipticity for both Ar and N2, and quantitatively depend on targets and trajectory paths. The experimental results are well reproduced by a nonadiabatic semiclassical simulation and explained by trajectory-based analysis. In addition, the influence of nuclear distance on the ratios is theoretically investigated. Our work reveals that the difference between atoms and molecules can be attributed to the influence of different ionic potentials, which depends on the molecular structure (internuclear distance) and alignment, on the evolution of the photoelectron.
Barnett W, Xiao X, Zhou Y. Competitive Exclusion vs. Mimetic Isomorphism? An Identified Empirical Test. Sociological Science [Internet]. 2021;8:211-219. 访问链接Abstract
Why are organizations sometimes so similar, and in other cases so different? For decades this question has been central to research on organizations, and two leading theories have answered the question very differently. Neo-institutional theory has pointed to the importance of mimetic isomorphism, where organizations imitate one another as they navigate decisions in the context of uncertainty over what is regarded as legitimate action. By contrast, ecological theory argues that competitive exclusion explains the differences we see around us, as organizations repel one another when they vie for the same resources. Decades of empirical work has tended to confirm one or the other theory, with scant effort being made to reconcile these conflicting predictions. Furthermore, much of the existing empirical work is limited to descriptive studies that make little or no attempt to empirically identify their findings, leaving the empirical record open to concerns over endogeneity. This paper conducts an identified empirical test, in a context where the two arguments make opposing predictions. In an analysis of auditor selection after the collapse of Arthur Andersen, we find evidence of competitive exclusion, but no evidence of mimetic isomorphism. Implications for the continued progress of organization theory are discussed.
Feng Y, Wang J, Wang Y, Helal S. Completing missing prevalence rates for multiple chronic diseases by jointly leveraging both intra-and inter-disease population health data correlations, in Proceedings of the Web Conference 2021.; 2021:183–193.
Li S, Wu P, Zhang K. Complex foam flow in series and parallel through multiscale porous media: Physical model interpretation. International Journal of Heat and Mass Transfer [Internet]. 2021;164:120628. 访问链接Abstract
Complex foam flows in series and parallel are investigated by means of a self-designed high-pressure high-temperature laboratory physical model. A total of twenty-two foam flow experiments were conducted in the porous media with a wide permeability range over two orders of magnitude. Specifically, fifteen single and seven dual foam flows in porous media with respective permeability range of 37−9705 mD and 41−7838 mD were performed to determine a series of physiochemical properties in terms of foam rheology, fluid profile and mobility control. For the foam flows in series, the overall gas saturation with process of foam injection is found to quickly increase within initial period but then tend to be stable. At the end of foam injection, the gas saturation curve could be clearly distinguished with permeability variances that a sharp rising range for permeability from 37 to 1233 mD while a quasi-stable range from 1233 to 9705 mD. Mobility reduction factor and apparent viscosity of the single flow cases are found to increase initially but in subsequent a decline with the permeability increase, whose maximum values were equal to 726.34 and 646.44 mPa•s at the permeability of 4386 mD. Moreover, the mobility curve basically performs as a U shape with three distinct periods: a sharp initial decrease period from 37 to 564 mD in subsequent of a second uniform mobility from 564 to 7309 and third increase period from 7309 to 9705 mD. On the other hand, for the foam flow in parallel, the profile control effect is determined to be favorable for a medium permeability ranging from 282 to 3855 mD but unfavorable for either lower- or higher-permeability cases. In the post-foam water injection period, the gas saturation for the single flow case monotonically decreases while for the flow in parallel, the gas and liquid production profiles perform oppositely to the profile control effect with respect to the permeability. Overall, gas and liquid mobilities are proven to be simultaneously controlled for foam flows in series and parallel through multiscale porous media, whereas a gas mobility is better controlled, particularly in porous media with lower permeability.
Yuan Y, Rezaee R, Yu H, Zou J, Liu K, Zhang Y. Compositional controls on nanopore structure in different shale lithofacies: A comparison with pure clays and isolated kerogens. Fuel [Internet]. 2021;303:121079. 访问链接Abstract
Nanopore structure development in shale is intimated with lithofacies that demonstrates a large variety in different formations. It is critical to differentiate and quantify the separate impact of lithological components (minerals and organic matter (OM)) on pore structure attributes associated with shale gas storage capacity. In this study, we classified shales into 12 lithofacies for compositional and petrophysical quantification. Parameters of our main target, the Goldwyer shales (argillaceous OM-poor, argillaceous OM-moderate, and argillaceous OM-rich lithofacies) were further compared with other shale lithofacies, pure clays and isolated kerogens, using XRD, Rock-Eval pyrolysis, Ar-SEM and low-pressure CO2/N2 gas adsorption techniques. Results show that argillaceous OM-rich lithofacies (TOC > 2% and illite-dominated clay contents > 50%) develop more interconnected pores with better hydrocarbon storage potential. The argillaceous lithofacies have large amounts of cleavage-sheet pores with large pore volumes; the accumulative pore volume of the pores in diameter from 2 to 17 nm constitutes the major amount of total pore volume that is associated with free gas. The OM-rich lithofacies develop more OM-pores (particularly in pore diameter <2 nm) that contain extraordinarily high specific surface area (SSA); the SSA of micropores makes up the major total surface area that is intimated with adsorbed gas. Further investigation on pure clays and isolated kerogens clarifies that illite mainly controls the pore sizes from 2 to 17 nm, resulting in large pore volumes in argillaceous shales. By contrast, isolated kerogen dominantly controls micropores in diameter <2 nm, leading to a larger surface area with higher adsorbed gas storage in organic-rich shales.
Zhao D, Liu W, Li F, Xu T, Zhu Y, Duan J, Wei Z.; 2021. Compositions and methods for removal of per- and polyfluoroalkyl substances (pfas). United States of America patent US US20210206670A1. 访问链接Abstract
The invention relates to composite compositions including a carbonaceous material and a photocatalyst. The invention includes compositions and various methods, including methods for removing one or more contaminants from a substance such as air, soil, and water.

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