科研成果

2021
Shang D, Peng JF, Guo S, Wu Z, Hu M*. Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China. Front. Environ. Sci. Eng. [Internet]. 2021;15(2):34. 访问链接
Chen Y, Zheng P, Wang Z, Pu W, Tan Y, Yu C, Xia M, Wang W, Guo J, Huang D, et al. Secondary Formation and Impacts of Gaseous Nitro-Phenolic Compounds in the Continental Outflow Observed at a Background Site in South China. Environmental Science & Technology [Internet]. 2021. 访问链接
Wang Y, Hu M, Hu W, Zheng J, Niu H, Fang X, Xu N, Wu Z, Guo S, Wu Y, et al. Secondary Formation of Aerosols Under Typical High-Humidity Conditions in Wintertime Sichuan Basin, China: A Contrast to the North China Plain. Journal of Geophysical Research: AtmospheresJournal of Geophysical Research: AtmospheresJournal of Geophysical Research: Atmospheres. 2021;126.Abstract
The Sichuan Basin is one of the regions suffering from severe haze pollution in southwest China. However, the secondary aerosol formation in this region is poorly understood. In this study, the chemical compositions of PM2.5 and molecular compositions of water-soluble organics in wintertime Sichuan were measured to investigate the aerosol sources and formation under typical high relative humidity (RH) conditions. Strong correlations between PM2.5, carbonaceous aerosols and K+ suggested the influence of biomass burning. The impacts of biomass burning were also supported by the dominance of primarily emitted reduced/less oxidized nitrogen-containing organics as well as the high peak intensities of secondarily formed nitrocatechols and methyl-nitrocatechols. High humidity (average RH = 80%) and aerosol liquid water (ALW) in Sichuan facilitated the secondary formation of sulfate, nitrate, and secondary organic aerosols (SOA). The average sulfate oxidation ratio and nitrogen oxidation ratio in Sichuan were 2.5 and 3.1 times of those in winter Beijing (average RH = 27%). This suggested higher potentials of SO2 and NOx to form sulfate and nitrate under high-RH conditions. The abundant aqueous-SOA formation in Sichuan was supported by the dominance of organosulfates (OSs) and nitrooxy-OSs in mass spectra of water-soluble organics, while the OSs in winter Beijing were quite limited. The more abundant OS formation in Sichuan was attributed to the much higher RH, ALW, aerosol acidity, and sulfate, which favored the acidic sulfate-catalyzed aqueous-phase reactions for OS formation. Higher concentrations of biogenic volatile organic compounds were additional reasons for the more abundant OSs in Sichuan than in Beijing. © 2021. American Geophysical Union. All Rights Reserved.
Liao K, Chen Q, Liu Y, Li Y, Lambe AT, Zhu T, Huang R-J, Zheng Y, Cheng X, Miao R, et al. Secondary Organic Aerosol Formation of Fleet Vehicle Emissions in China: Potential Seasonality of Spatial Distributions. Environmental Science & Technology. 2021;55(11):7276-7286.
Zhang Z, Zhu W, Hu M*, Wang H, Chen Z, Shen R, Yu Y, Tan R, Guo S. Secondary Organic Aerosol from Typical Chinese Domestic Cooking Emissions. Environmental Science and Technology Letters [Internet]. 2021;8(1):24–31. 访问链接Abstract
Cooking has been proven to be a significant source of primary organic aerosol, especially in megacities. However, the formation of secondary organic aerosol (SOA) derived from cooking emissions is still poorly understood. In this work, four prevalent Chinese domestic cooking types involving complicated cuisines and various cooking methods were chosen to conduct a lab simulation for SOA formation using a Gothenburg potential aerosol mass reactor (Go: PAM). After samples had been aged under OH exposures of 4.3–27.1 × 1010 molecules cm–3 s, the domestic cooking SOA was characterized by mass growth potentialities (1.81–3.16), elemental ratios (O/C = 0.29–0.41), and mass spectra. Compared with other organic aerosol (OA), domestic cooking SOA is a kind of less oxidized oxygenated OA (LO-OOA) with a unique oxidation pathway (alcohol/peroxide pathway) and mass spectra (characteristic peaks at m/z 28, 29, 41, 43, 44, 55, and 57). This study is expected to identify the cooking SOA under actual cooking conditions, which could contribute to the formulation of pollution source control as well as the health risk assessment of exposure to cooking fumes.
Zhang Z, Zhu W, Hu M, Wang H, Chen Z, Shen R, Yu Y, Tan R, Guo S. Secondary Organic Aerosol from Typical Chinese Domestic Cooking Emissions. Environmental Science and Technology LettersEnvironmental Science and Technology LettersEnvironmental Science and Technology Letters. 2021;8:24-31.Abstract
Cooking has been proven to be a significant source of primary organic aerosol, especially in megacities. However, the formation of secondary organic aerosol (SOA) derived from cooking emissions is still poorly understood. In this work, four prevalent Chinese domestic cooking types involving complicated cuisines and various cooking methods were chosen to conduct a lab simulation for SOA formation using a Gothenburg potential aerosol mass reactor (Go: PAM). After samples had been aged under OH exposures of 4.3-27.1 × 1010 molecules cm-3 s, the domestic cooking SOA was characterized by mass growth potentialities (1.81-3.16), elemental ratios (O/C = 0.29-0.41), and mass spectra. Compared with other organic aerosol (OA), domestic cooking SOA is a kind of less oxidized oxygenated OA (LO-OOA) with a unique oxidation pathway (alcohol/peroxide pathway) and mass spectra (characteristic peaks at m/z 28, 29, 41, 43, 44, 55, and 57). This study is expected to identify the cooking SOA under actual cooking conditions, which could contribute to the formulation of pollution source control as well as the health risk assessment of exposure to cooking fumes. ©
Cheng X, Chen Q, Li Y, Huang G, Liu Y, Lu S, Zheng Y, Qiu W, Lu K, Qiu X, et al. Secondary Production of Gaseous Nitrated Phenols in Polluted Urban Environments. Environmental Science & Technology. 2021;55(8):4410-4419.
Cheng X, Chen Q, Li Y, Huang G, Liu Y, Lu S, Zheng Y, Qiu W, Lu K, Qiu X, et al. Secondary Production of Gaseous Nitrated Phenols in Polluted Urban Environments. Environmental Science & Technology [Internet]. 2021:null. 访问链接
Schuller F, Urquhart J  S, Csengeri T, Colombo D, Duarte-Cabral A, Mattern M, Ginsburg A, Pettitt A  R, Wyrowski F, Anderson L, et al. The SEDIGISM survey: First Data Release and overview of the Galactic structure. \mnras. 2021;500:3064-3082.
Duarte-Cabral A, Colombo D, Urquhart J  S, Ginsburg A, Russeil D, Schuller F, Anderson L  D, Barnes P  J, Beltrán M  T, Beuther H, et al. The SEDIGISM survey: molecular clouds in the inner Galaxy. MNRAS [Internet]. 2021;500:3027-3049. 访问链接
Zuo K, Wang K, DuChanois RM, Fang Q, Deemer EM, Huang X, Xin R, Said IA, He Z, Feng Y, et al. Selective membranes in water and wastewater treatment: Role of advanced materials. Materials Today. 2021.Abstract
Membrane separation has enjoyed tremendous advances in relevant material and engineering sciences, making it the fastest growing technology in water treatment. Although membranes as a broad-spectrum physical barrier have great advantages over conventional treatment processes in a myriad of applications, the need for higher selectivity and specificity in membrane separation is rising as we move to target contaminants at trace concentrations and to recover valuable chemicals from wastewater with low energy consumption. In this review, we discuss the drivers, fundamental science, and potential enabling materials for high selectivity membranes, as well as their applications in different water treatment processes. Membrane materials and processes that show promise to achieve high selectivity for water, ions, and small molecules—as well as the mechanisms involved—are highlighted. We further identify practical needs, knowledge gaps, and technological barriers in both material development and process design for high selectivity membrane processes. Finally, we discuss research priorities in the context of existing and future water supply paradigms.
Zhang Y, Xu L, Liu Z, Cui X, Xiang Z, Bai J, Jiang D, Xue J, Wang C, Lin Y. Self-powered pulsed direct current stimulation system for enhancing osteogenesis in MC3T3-E1. Nano Energy. 2021;85:106009.
Ouyang H, Jiang D, Fan Y, Wang ZL, Li Z. Self-powered technology for next-generation biosensor. Science bulletin. 2021;66(17):1709-1712.
Yang Y, Xu L, Jiang D, Chen BZ, Luo R, Liu Z, Qu X, Wang C, Shan Y, Cui Y. Self‐powered controllable transdermal drug delivery system. Advanced Functional Materials. 2021;31(36):2104092.
Huang Y, Mill L, Stoll R, Kling L, Aust O, Wagner F, Grüneboom A, Schett G, Christiansen S, Maier A. Semi-permeable filters for interior region of interest dose reduction in X-ray microscopy, in Bildverarbeitung für die Medizin 2021: Proceedings, German Workshop on Medical Image Computing, Regensburg, March 7-9, 2021. Springer Fachmedien Wiesbaden Wiesbaden; 2021:61–66.
Zeng XW, Hu* YF. Sensation and Perception of a Bioinspired Flexible Smart Sensor System. ACS Nano. 2021;15:9238.
Zeng XW, Hu* YF. Sensation and Perception of a Bioinspired Flexible Smart Sensor System. ACS Nano. 2021;15:9238.
Fan L, Kong L, Li L, Qu T. Sensitivity to a break in interaural correlation in frequency-gliding noises. Front. Psychol. - Perception Science. 2021.
Shi Y, Han Y, Wang Y, Qi L, Chen X, Chen W, Li W, Zhang H, Zhu T, Gong J. Serum branched-chain amino acids modifies the associations between air pollutants and insulin resistance. Ecotoxicology and Environmental SafetyEcotoxicology and Environmental Safety. 2021;225.
董春涛, 沈晴霓, 罗武, 吴鹏飞, 吴中海. SGX应用支持技术研究进展. 软件学报. 2021;32(1):137-166.

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