科研成果

2021
Zheng ZJ, Kulasegaram S, Chen P, Chen YQ. An efficient SPH methodology for modelling mechanical characteristics of particulate composites. Defence TechnologyDefence Technology. 2021;17:135-146.Abstract
Particulate composites are one of the widely used materials in producing numerous state-of-the-art components in biomedical, automobile, aerospace including defence technology. Variety of modelling techniques have been adopted in the past to model mechanical behaviour of particulate composites. Due to their favourable properties, particle-based methods provide a convenient platform to model failure or fracture of these composites. Smooth particle hydrodynamics (SPH) is one of such methods which demonstrate excellent potential for modelling failure or fracture of particulate composites in a Lagrangian setting. One of the major challenges in using SPH method for modelling composite materials depends on accurate and efficient way to treat interface and boundary conditions. In this paper, a master-slave method based multi-freedom constraints is proposed to impose essential boundary conditions and interfacial displacement constraints in modelling mechanical behaviour of composite materials using SPH method. The proposed methodology enforces the above constraints more accurately and requires only smaller condition number for system stiffness matrix than the procedures based on typical penalty function approach. A minimum cut-off value-based error criteria is employed to improve the computational efficiency of the proposed methodology. In addition, the proposed method is further enhanced by adopting a modified numerical interpolation scheme along the boundary to increase the accuracy and computational efficiency. The numerical examples demonstrate that the proposed master-slave approach yields better accuracy in enforcing displacement constraints and requires approximately the same computational time as that of penalty method. (C) 2020 China Ordnance Society. Production and hosting by Elsevier B.V. on behalf of KeAi Communications Co.
Yang Y, Li X, Zu K, Lian C, Chen S, Dong HB, Feng M, Liu H, Liu J, Lu K, et al. Elucidating the effect of HONO on O-3 pollution by a case study in southwest China. Science of the Total Environment [Internet]. 2021;756. 访问链接
Yu Y, Wang H, Wang T, Song K, Tan T, Wan Z, Gao Y, Dong H, Chen S, Zeng L, et al. Elucidating the importance of semi-volatile organic compounds to secondary organic aerosol formation at a regional site during the EXPLORE-YRD campaign. Atmospheric EnvironmentAtmospheric EnvironmentAtmospheric Environment. 2021;246.Abstract
To investigate the regional secondary organic aerosol (SOA) formation at Yangtze River Delta (YRD) region, China, the chemical composition of fine particles and their gaseous precursors were simultaneously measured at a regional site, Taizhou, during EXPeriment on the eLucidation of the atmospheric Oxidation capacity, aerosol foRmation and their Effects in Yangtze River Delta (EXPLORE-YRD) intensive field campaign from May to June 2018. Secondary organic carbon (SOC) was estimated by both bottom-up and top-down method, i.e. the yield method from volatile organic compounds (VOCs) oxidation, and the elemental carbon (EC) tracer method. Our result showed that the oxidation of alkanes and aromatics measured by GC-MS/FID based on the yield method could only explain 25.3% of the SOC derived from the EC tracer method, in which aromatics were the dominant contributors (23.9%). This percentage increased to 39.5% while two semi-volatile organic compounds (SVOCs), i.e. naphthalene, and methylnaphthalene, were used in the calculation, suggesting the importance of SVOCs on SOA formation. The SOA formation pathways were further explored. The good correlation of SOC and odd oxygen (Ox) indicated the important role of photochemical reactions on SOA formation in the summer of YRD. Our findings evaluated the contributions of VOCs to SOA formation in Taizhou, revealed the importance of SVOCs to SOA formation and highlighted an urgent need for more exploration of SVOCs in the future. © 2020 The Authors
Liu Z, Wang Y, Hu B, Lu K, Tang G, Ji D, Yang X, Gao W, Xie Y, Liu J, et al. Elucidating the quantitative characterization of atmospheric oxidation capacity in Beijing, China. Science of the Total Environment [Internet]. 2021;771. 访问链接
Wang T*, Huang T, Jiang H, Ma R. Electrochemical degradation of atrazine by BDD anode: Evidence from compound-specific stable isotope analysis and DFT simulations. Chemosphere. 2021;273:129754.
Ji G, Shi J. Emergence of Dirac composite fermions: Dipole picture. Phys. Rev. Research [Internet]. 2021;3:043055. 访问链接
Wu L, Wang Z, Wang B, Chen Q, Bao L, Yu Z, Yang Y, Ling Y, Qin Y, Tang K, et al. Emulation of biphasic plasticity in retinal electrical synapses for light-adaptive pattern pre-processing. Nanoscale [Internet]. 2021;13:3483-3492. 访问链接Abstract
Electrical synapses provide rapid, bidirectional communication in nervous systems, accomplishing tasks distinct from and complementary to chemical synapses. Here, we demonstrate an artificial electrical synapse based on second-order conductance transition (SOCT) in an Ag-based memristor for the first time. High-resolution transmission electron microscopy indicates that SOCT is mediated by the virtual silver electrode. Besides the conventional chemical synaptic behaviors, the biphasic plasticity of electrical synapses is well emulated by integrating the device with a photosensitive element to form an optical pre-processing unit (OPU), which contributes to the retinal neural circuitry and is adaptive to ambient illumination. By synergizing the OPU and spiking neural network (SNN), adaptive pattern recognition tasks are accomplished under different light and noise settings. This work not only contributes to the further completion of synaptic behaviour for hardware-level neuromorphic computing, but also potentially enables image pre-processing with light adaptation and noise suppression for adaptive visual recognition.
Wu L, Bao L, Wang Z, Yu Z, Wang B, Chen Q, Ling Y, Qin Y, Tang K, Cai Y, et al. Emulation of Synaptic Scaling Based on MoS2 Neuristor for Self-Adaptative Neuromorphic Computing. Advanced Electronic Materials [Internet]. 2021;7:2001104. 访问链接Abstract
Abstract Recent studies indicate that synaptic scaling is a vital mechanism to solve instability risks brought by the positive feedback of synaptic weight change related with standalone Hebbian plasticity. There are two kinds of synaptic scaling in the neural network, including local scaling and global scaling, both important for stabilizing the neural function. In this paper, for the first time, local synaptic scaling is emulated based on the MoS2 neuristor. The first-principle calculation reveals that synaptic scaling achieved by the neuristor is associated with an internal residual Li+-related weak dynamical process. Experimental results show the potential of achieving global synaptic scaling by the same device. Moreover, inspired by the synaptic scaling in the human brain, a new method of weight mapping called weight scaling mapping (WSM) is proposed to improve the stability of an artificial neural network (ANN). The simulation results indicate that WSM can improve the accuracy and anti-noise ability of the network compared with the traditional mapping method. These findings provide new insight into bionic research and help advance the construction of stable neuromorphic systems.
Wu L, Bao L, Wang Z, Yu Z, Wang B, Chen Q, Ling Y, Qin Y, Tang K, Cai Y, et al. Emulation of Synaptic Scaling Based on MoS2 Neuristor for Self-Adaptative Neuromorphic Computing. Advanced Electronic Materials. 2021:2001104.
王延飞,杜元清著. 情报感知论. 北京: 科学技术文献出版社; 2021.Abstract
      本书作者在长期科技情报研究工作实践与理论探索中深刻感受到明辨情报工作的使命本质、探究情报业务的特殊要求何其重要!在国家社科基金项目支持下,本书从情报任务种类和流程区分入手,探析情报感知的规律和规范,试图由此而找到可以用于分析中国情报学术和情报事业发展的理念和工具。
Jia J, Shibata T, Xie J, Zhang D-Q. Endomorphisms of quasi-projective varieties -- towards Zariski dense orbit and Kawaguchi-Silverman conjectures. [Internet]. 2021. pdf
Luo J, Xu W, Du Y, Fu B, SONG J, Fu Z, Yang M, Li Y, Ye L, Huang Q. Energy-and area-efficient Fe-FinFET-based time-domain mixed-signal computing in memory for edge machine learning. 2021 IEEE International Electron Devices Meeting (IEDM). 2021:19.5. 1-19.5. 4.
Li H, Tan Z, Bao Y, Xiao H, Zhang H, Du K, Shen L, Ru J, Zhang Y, Ye L, et al. Energy-Efficient CMOS Humidity Sensors Using Adaptive Range-Shift Zoom CDC and Power-Aware Floating Inverter Amplifier Array. IEEE Journal of Solid-State Circuits. 2021;56:3560-3572.Abstract
This article presents an adaptive zoom-capacitance-to-digital converter (CDC)-based CMOS humidity sensor. The humidity sensor is realized by means of two differential capacitors whose dielectrics are sensitive to humidity. The sensing capacitors are interfaced with a zoom CDC, which consists of a successive-approximation-register (SAR) analog-to-digital converter (ADC) and a 3rd-order delta–sigma modulator ( $Δ Σ \textM$ ). The SAR ADC eliminates the influence of the baseline capacitance to reduce the input range of the $Δ Σ \textM$ . To improve the energy efficiency of the CDC across the full input range, a power-aware floating inverter amplifier (FIA) array is proposed, which is configured based on the conversion results of the SAR logic. In addition, an adaptive range-shift (ARS) zoom CDC is proposed to: 1) resist off-chip parasitics and interference and 2) allow low redundancy and a more energy-efficient FIA-based comparator, thus reducing power consumption. The proposed CMOS humidity sensor is implemented in a 0.11- $μ \textm$ CMOS process. Measurement results show a capacitance resolution of 17.9 aF and an effective number of bits (ENOB) of 14.0 within a conversion time of 1.01 ms. The proposed humidity sensor consumes 1.5 $μ \textW$ of power and exhibits a 0.0094 % relative humidity (RH) resolution and a ±1.5 %RH peak-to-peak accuracy (3 $\sigma $ error of 5.5 %RH) among 12 chips from 20 to 85 %RH, and it achieves a figure of merit (FoM) of 0.135 pJ $\cdot $ %RH2, which is more than six times better than the state of the art.
Yu M, Li Y, Yang W, Yuan X, Li N, He W, Feng Y, Liu J. Enhanced electrocatalytic activity and antifouling performance by iron phthalocyanine doped filtration membrane cathode. Chemical Engineering Journal. 2021;413:127536.
Yu M, Li Y, Yang W, Yuan X, Li N, He W, Feng Y, Liu J. Enhanced electrocatalytic activity and antifouling performance by iron phthalocyanine doped filtration membrane cathode. Chemical Engineering Journal. 2021;413:127536.
Wang Y, Huang D, Huang W, Liu B, Chen Q, Huang R, Gen M, Mabato BRG, Chan CK, Li X, et al. Enhanced Nitrite Production from the Aqueous Photolysis of Nitrate in the Presence of Vanillic Acid and Implications for the Roles of Light-Absorbing Organics. Environmental Science & Technology [Internet]. 2021. 访问链接
Zong Y, Shao Y, Zeng Y, Shao B, Xu L, Zhao Z, Liu W, Wu D. Enhanced Oxidation of Organic Contaminants by Iron(II)-Activated Periodate: The Significance of High-Valent Iron–Oxo Species. Environmental Science & Technology [Internet]. 2021;55:7634-7642. 访问链接Abstract
Potassium periodate (PI, KIO4) was readily activated by Fe(II) under acidic conditions, resulting in the enhanced abatement of organic contaminants in 2 min, with the decay ratios of the selected pollutants even outnumbered those in the Fe(II)/peroxymonosulfate and Fe(II)/peroxydisulfate processes under identical conditions. Both 18O isotope labeling techniques using methyl phenyl sulfoxide (PMSO) as the substrate and X-ray absorption near-edge structure spectroscopy provided conclusive evidences for the generation of high-valent iron–oxo species (Fe(IV)) in the Fe(II)/PI process. Density functional theory calculations determined that the reaction of Fe(II) with PI followed the formation of a hydrogen bonding complex between Fe(H2O)62+ and IO4(H2O)−, ligand exchange, and oxygen atom transfer, consequently generating Fe(IV) species. More interestingly, the unexpected detection of 18O-labeled hydroxylated PMSO not only favored the simultaneous generation of ·OH but also demonstrated that ·OH was indirectly produced through the self-decay of Fe(IV) to form H2O2 and the subsequent Fenton reaction. In addition, IO4– was not transformed into the undesired iodine species (i.e., HOI, I2, and I3–) but was converted to nontoxic iodate (IO3–). This study proposed an efficient and environmental friendly process for the rapid removal of emerging contaminants and enriched the understandings on the evolution mechanism of ·OH in Fe(IV)-mediated processes.
Yu M, Yang W, Yuan X, Li Y, Li N, He W, Feng Y, Liu J. Enhanced oxygen reduction activity and high-quality effluent of membrane filtration electrodes with Prussian blue in microbial fuel cells. Science of The Total Environment. 2021;753:142021.
Yu M, Yang W, Yuan X, Li Y, Li N, He W, Feng Y, Liu J. Enhanced oxygen reduction activity and high-quality effluent of membrane filtration electrodes with Prussian blue in microbial fuel cells. Science of The Total Environment. 2021;753:142021.
Zhou Q, Sun H, Jia L, Zhao L, Wu W. Enhanced pollutant removal from rural non-point source wastewater using a two-stage multi-soil-layering system with blended carbon sources: Insights into functional genes, microbial community structure and metabolic function. CHEMOSPHERE. 2021;275.Abstract
A two-stage multi-soil-layering system with blended carbon sources (MSL-BCS) was constructed at pilot scale for treatment of rural non-point source wastewater. Results showed the MSL-BCS system had effective removal efficiencies with 64% of TN and 60% of TP, respectively. The addition of BCS could result in higher (1.6-3.1 fold) denitrification gene abundances (nirS and nosZ) for enhancing denitrification. High-throughput sequencing approach revealed that the higher abundance (>50%) of Epsilonbacteraeotra (Genus: Sulfuricurvum, Family: Thiovulaceae, Class: Campylobacteria, Phylum: Epsilonbacteraeota) enriched in the surface of BCS, which suggested that Epsilonbacteraeotra are the keystone species in achieving nitrogen removal through enhancing denitrification at oligotrophic level. KEGG analysis indicated that BCS might release some signaling molecules for enhancing the energy metabolism process, as well as stimulate the enzyme activities of histidine kinase, glycogen phosphorylase and ATPase, and thereby the denitrification processes were strengthened in MSL-BCS system. Consequently, this study could provide some valuable information on the removal performance and mechanism of engineering MSL systems packed with BCS to govern the rural wastewater treatment. (C) 2021 Elsevier Ltd. All rights reserved.

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