科研成果

2021
Gongbuzeren, Li WJ, Lai YP. The Role of Community Cooperative Institutions in Building Rural–Urban Linkages Under Urbanization of Pastoral Regions in China. Frontiers in Sustainable Food Systems [Internet]. 2021;(4). 访问链接Abstract
In contrast to agricultural settings, the process of urbanization in the pastoral regions of China are largely driven by long-term influences of ecological conservation and the provision of social services. Consequently, many of the herders who have migrated into nearby secondary urban centers depend on resources from pastoral regions to support their livelihoods, forming complex patterns of rural–urban linkages. While current literature has discussed the processes of herder out-migration and their implications on rural and urban livelihood development, few studies have examined the linkages between the herders living in the pastoral regions and those who have out-migrated to urban regions and their importance in rural livelihood transformation. Based on past studies, we argue that, in a changing pastoral social–ecological system, herders living in both rural and urban regions depend on each other to support their livelihoods through three types of mobility: (1) livestock mobility, (2) herder mobility, and (3) resource mobility. However, what innovative institutions in rangeland resource management and herder economic cooperation can do to help maintain these three types of mobility to sustain rural livelihood development, becomes a critical challenge. Innovative community cooperative institutions developed by pastoral communities from the Tibetan Plateau and Inner Mongolia may be able to offer new perspective and insight on how to better maintain rural–urban linkages in the processes of urbanization in pastoral regions. In this current study will present the two cases of innovative institutions and the roles they play in facilitating the three types of mobility to address livelihood challenges. While current studies recommend an increase of government subsidies, provision of vocational training, and social insurance that help herders better adapt to urban livelihood, we argue that rangeland management and community economic cooperation in innovative institutions are needed to facilitate the mobility of livestock, resources, and the herder population, and maybe only then the livelihood challenges that migrated herders are facing will be addressed effectively.
Wei* Y, Evers-Vermeul J, Sanders TJM, Mak WM. The role of connectives and stance markers in the processing of subjective causal relations. Discourse Processes [Internet]. 2021. Full textAbstract
Interpreting subjectivity in causal relations takes effort: Subjective, claim-argument relations are read slower than objective, cause-consequence relations. In an eye-tracking-while-reading experiment, we investigated whether connectives and stance markers can play a facilitative role. Sixty-five Chinese participants read sentences expressing a subjective causal relation, systematically varied in the use of stance markers (no, attitudinal, epistemic) in the first clause and connectives (neutral suoyi “so”, subjective kejian “so”) in the second clause. Results showed that processing subjectivity proceeds highly incrementally: The interplay of the subjectivity markers is visible as the sentence unfolds. Subjective connectives increased reading times, irrespective of the type of stance marker being used. Stance markers did, however, facilitate the processing of modal verbs in subjective relations. We conclude that processing subjectivity involves evaluating how the argument supports the claim and that connectives, modal verbs, and stance markers function as processing instructions that help readers achieve this evaluation.
Ou Y, Iyer G, Binsted M, Patel P, Kim S, Wise M. Role of energy storage in US capacity expansion pathways with improved modeling of power sector dynamics. AGU Fall Meeting Abstracts. 2021;2021:GC25M-0789.
Fuhrman J, Clarens AF, McJeon H, Patel P, Ou Y, Doney SC, Shobe WM, Pradhan S. The role of negative emissions in meeting China’s 2060 carbon neutrality goal. Oxford Open Climate Change. 2021;1(1):kgab004.
ZOU C, CUI X, KUANG Y, LIU K, Wang Y, WANG X, HUANG R. A Scatter-and-Gather Spiking Convolutional Neural Network on a Reconfigurable Neuromorphic Hardware. Frontiers in Neuroscience. 2021;15:694170.Abstract
Artificial neural networks (ANNs), like convolutional neural networks (CNNs), have achieved the state-of-the-art results formanymachine learning tasks. However, inference with large-scale full-precision CNNs must cause substantial energy consumption and memory occupation, which seriously hinders their deployment on mobile and embeddedsystems. Highly inspired from biological brain, spiking neural networks (SNNs) are emerging as new solutions because of natural superiority in brain-like learning and great energy efficiency with event-driven communication and computation. Nevertheless, training a deep SNN remains a main challenge and there is usually a big accuracy gap between ANNs and SNNs. In this paper, we introduce a hardware-friendly conversion algorithm called “scatter-and-gather” to convert quantized ANNs to lossless SNNs, where neurons are connected with ternary {−1,0,1} synaptic weights. Each spiking neuron is stateless and more like original McCulloch and Pitts model, because it fires at most one spike and need be reset at each time step. Furthermore, we develop an incremental mapping framework to demonstrate efficient network deployments on a reconfigurable neuromorphic chip. Experimental results show our spiking LeNet on MNIST and VGG-Net on CIFAR-10 datasetobtain 99.37% and 91.91% classification accuracy, respectively. Besides, the presented mapping algorithm manages network deployment on our neuromorphic chip with maximum resource efficiency and excellent flexibility. Our four-spike LeNet and VGG-Net on chip can achieve respective real-time inference speed of 0.38 ms/image, 3.24 ms/image, and an average power consumption of 0.28 mJ/image and 2.3 mJ/image at 0.9 V, 252 MHz, which is nearly two orders of magnitude more efficient than traditional GPUs.
Liu X-C, Wu Y, Zhang C, Chen X, Lin L-H, Qin S-L, Liu T, Henkel C, Wang J, Liu H-L, et al. A Search for Cloud Cores Affected by Shocked Carbon Chain Chemistry in L1251. \apj. 2021;912:148.
Sun M, Zhou Y, Wang Y, Zheng X, Cui J, Zhang D, Zhang J, Zhang R. Seasonal discrepancies in peroxyacetyl nitrate (PAN) and its correlation with ozone and PM2.5: Effects of regional transport from circumjacent industrial cities. Science of the Total Environment [Internet]. 2021;785. 访问链接Abstract
Peroxyacetyl nitrate (PAN) is the most important reservoir of nitrogen oxides, with effects on atmospheric oxidation capacity and regional nitrogen distribution. The first yearlong observational study of PAN was conducted from September 2018 to August 2019 at a suburban site and an urban site in Zhengzhou, Henan Province, central China. Compared with studies over the past two decades, summer PAN pollution at the suburban site and winter PAN pollution at both sites were more significant, with annual average concentrations of 1.96 ± 1.44 and 2.01 ± 1.59 ppbv, respectively. Seasonal PAN discrepancies between the urban and suburban areas were analyzed in detail. Active PAN formation, regional transport, photochemical precursors, and PAN lifetime played key roles during seasons with elevated PAN (winter and spring). According to the results of cluster analysis and potential source contribution function analysis, during the cold months, short-distance air mass transport from the east, south, and southeast of Henan Province and southern Hebei Province increased PAN pollution in urban Zhengzhou. PAN source areas were located in circumjacent industrial cities surrounding Zhengzhou except in the northeastern direction. Based on the relationships between pollutant concentrations, wind speed, and wind direction, a strong positive correlation between PAN and PM2.5 (and O3) existed in winter due to their joint transport. A slow-moving, low-height air mass passed through surrounding industrial cities before reaching the study area, carrying both pollutants and leading to strong consistency between PAN and O3 levels. The long-term PAN characteristics described in this study will help clarify the causes of regional air pollution in inland city agglomerations. Moreover, the PAN correlations and joint transport of PAN and PM2.5 (or O3) support the use of PAN as an indicator of air pollution introduced from surrounding industrial areas. © 2021 Elsevier B.V.
Deng H, Guan B, Wang J, Zuo A, Wang Z, Sun T. Seasonal Land Fallowing Policy in Response to Groundwater Overdraft in the North China Plain. Water Alternatives. 2021;14.
Zhu W, Zhou M, Cheng Z, Yan N, Huang C, Qiao L, Wang H, Liu Y, Lou S, Guo S. Seasonal variation of aerosol compositions in Shanghai, China: Insights from particle aerosol mass spectrometer observations. Science of the Total EnvironmentScience of the Total Environment. 2021;771.Abstract
The variations of non-refractory submicron aerosol (NR-PM1) were characterized using an high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and other online instruments measurements sampled at an urban site in Shanghai from 2016 to 2017. Spring (from 18 May to 4 June 2017), summer (from 23 August to 10 September 2017) and winter (from 28 November 2016 to 23 January 2017) seasons were chosen for detail investigating the seasonal variations in the aerosol chemical characteristics. The average PM1 (NR-PM1 + BC) mass concentration showed little difference in the three seasons in Shanghai. The average mass concentrations of total PM1 during spring, summer, and winter observations in Shanghai were 23.9 ± 20.7 μg/m3, 28.5 ± 17.6 μg/m3, and 31.9 ± 22.7 μg/m3, respectively. The seasonal difference on chemical compositions was more significant between them. Organic aerosol (OA) and sulfate were dominant contributor of PM1 in summer, whereas OA and nitrate primarily contribution to the increase of PM1 mass loading in spring and winter. As an abundant component in PM1 (accounting for 39%–49%), OA were resolved into two primary organic aerosol (POA) factors and two secondary aerosol (SOA) factors by using positive matrix factorization (PMF), of which OA was overwhelmingly dominated by the SOA (50–60%) across the three seasons in Shanghai. Correlation analysis with relative humidity and odd oxygen indicated that aqueous-phase processing and played an important role in more aged SOA formation in summer and winter. In spring, both aqueous-phase and photochemical processing contributed significantly to fresh SOA formation. Our results suggest the significant role of secondary particles in PM pollution in Shanghai and highlight the importance of control measures for reducing emissions of gaseous precursors, especially need to consider seasonal characteristics. © 2021 Elsevier B.V.
Shang D, Peng JF, Guo S, Wu Z, Hu M*. Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China. Front. Environ. Sci. Eng. [Internet]. 2021;15(2):34. 访问链接
Shang D, Peng J, Guo S, Wu Z, Hu M. Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China. Frontiers of Environmental Science and EngineeringFrontiers of Environmental Science and EngineeringFrontiers of Environmental Science and Engineering. 2021;15.Abstract
Severe haze pollution occurs frequently in the winter over the Beijing-Tianjin-Hebei (BTH) region (China), exerting profound impacts on air quality, visibility, and human health. The Chinese Government has taken strict mitigation actions since 2013 and has achieved a significant reduction in the annual mean PM2.5 concentration over this region. However, the level of secondary aerosols during heavy haze episodes showed little decrease during this period. During heavy haze episodes, the concentrations of secondary aerosol components, including sulfate, nitrate and secondary organics, in aerosol particles increase sharply, acting as the main contributors to aerosol pollution. To achieve effective control of particle pollution in the BTH region, the precise and complete secondary aerosol formation mechanisms have been investigated, and advances have been made about the mechanisms of gas phase reaction, nucleation and heterogeneous reactions in forming secondary aerosols. This paper reviews the research progress in aerosol chemistry during haze pollution episodes in the BTH region, lays out the challenges in haze formation studies, and provides implications and directions for future research. [Figure not available: see fulltext.]. © 2020, Higher Education Press.
Shang D, Peng J, Guo S, Wu Z, Hu M. Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China. Frontiers of Environmental Science and EngineeringFrontiers of Environmental Science and Engineering. 2021;15.Abstract
Severe haze pollution occurs frequently in the winter over the Beijing-Tianjin-Hebei (BTH) region (China), exerting profound impacts on air quality, visibility, and human health. The Chinese Government has taken strict mitigation actions since 2013 and has achieved a significant reduction in the annual mean PM2.5 concentration over this region. However, the level of secondary aerosols during heavy haze episodes showed little decrease during this period. During heavy haze episodes, the concentrations of secondary aerosol components, including sulfate, nitrate and secondary organics, in aerosol particles increase sharply, acting as the main contributors to aerosol pollution. To achieve effective control of particle pollution in the BTH region, the precise and complete secondary aerosol formation mechanisms have been investigated, and advances have been made about the mechanisms of gas phase reaction, nucleation and heterogeneous reactions in forming secondary aerosols. This paper reviews the research progress in aerosol chemistry during haze pollution episodes in the BTH region, lays out the challenges in haze formation studies, and provides implications and directions for future research. [Figure not available: see fulltext.]. © 2020, Higher Education Press.
Chen Y, Zheng P, Wang Z, Pu W, Tan Y, Yu C, Xia M, Wang W, Guo J, Huang D, et al. Secondary Formation and Impacts of Gaseous Nitro-Phenolic Compounds in the Continental Outflow Observed at a Background Site in South China. Environmental Science & Technology [Internet]. 2021. 访问链接
Wang Y, Hu M, Hu W, Zheng J, Niu H, Fang X, Xu N, Wu Z, Guo S, Wu Y, et al. Secondary Formation of Aerosols Under Typical High-Humidity Conditions in Wintertime Sichuan Basin, China: A Contrast to the North China Plain. Journal of Geophysical Research: AtmospheresJournal of Geophysical Research: AtmospheresJournal of Geophysical Research: Atmospheres. 2021;126.Abstract
The Sichuan Basin is one of the regions suffering from severe haze pollution in southwest China. However, the secondary aerosol formation in this region is poorly understood. In this study, the chemical compositions of PM2.5 and molecular compositions of water-soluble organics in wintertime Sichuan were measured to investigate the aerosol sources and formation under typical high relative humidity (RH) conditions. Strong correlations between PM2.5, carbonaceous aerosols and K+ suggested the influence of biomass burning. The impacts of biomass burning were also supported by the dominance of primarily emitted reduced/less oxidized nitrogen-containing organics as well as the high peak intensities of secondarily formed nitrocatechols and methyl-nitrocatechols. High humidity (average RH = 80%) and aerosol liquid water (ALW) in Sichuan facilitated the secondary formation of sulfate, nitrate, and secondary organic aerosols (SOA). The average sulfate oxidation ratio and nitrogen oxidation ratio in Sichuan were 2.5 and 3.1 times of those in winter Beijing (average RH = 27%). This suggested higher potentials of SO2 and NOx to form sulfate and nitrate under high-RH conditions. The abundant aqueous-SOA formation in Sichuan was supported by the dominance of organosulfates (OSs) and nitrooxy-OSs in mass spectra of water-soluble organics, while the OSs in winter Beijing were quite limited. The more abundant OS formation in Sichuan was attributed to the much higher RH, ALW, aerosol acidity, and sulfate, which favored the acidic sulfate-catalyzed aqueous-phase reactions for OS formation. Higher concentrations of biogenic volatile organic compounds were additional reasons for the more abundant OSs in Sichuan than in Beijing. © 2021. American Geophysical Union. All Rights Reserved.
Liao K, Chen Q, Liu Y, Li Y, Lambe AT, Zhu T, Huang R-J, Zheng Y, Cheng X, Miao R, et al. Secondary Organic Aerosol Formation of Fleet Vehicle Emissions in China: Potential Seasonality of Spatial Distributions. Environmental Science & Technology. 2021;55(11):7276-7286.
Zhang Z, Zhu W, Hu M*, Wang H, Chen Z, Shen R, Yu Y, Tan R, Guo S. Secondary Organic Aerosol from Typical Chinese Domestic Cooking Emissions. Environmental Science and Technology Letters [Internet]. 2021;8(1):24–31. 访问链接Abstract
Cooking has been proven to be a significant source of primary organic aerosol, especially in megacities. However, the formation of secondary organic aerosol (SOA) derived from cooking emissions is still poorly understood. In this work, four prevalent Chinese domestic cooking types involving complicated cuisines and various cooking methods were chosen to conduct a lab simulation for SOA formation using a Gothenburg potential aerosol mass reactor (Go: PAM). After samples had been aged under OH exposures of 4.3–27.1 × 1010 molecules cm–3 s, the domestic cooking SOA was characterized by mass growth potentialities (1.81–3.16), elemental ratios (O/C = 0.29–0.41), and mass spectra. Compared with other organic aerosol (OA), domestic cooking SOA is a kind of less oxidized oxygenated OA (LO-OOA) with a unique oxidation pathway (alcohol/peroxide pathway) and mass spectra (characteristic peaks at m/z 28, 29, 41, 43, 44, 55, and 57). This study is expected to identify the cooking SOA under actual cooking conditions, which could contribute to the formulation of pollution source control as well as the health risk assessment of exposure to cooking fumes.
Zhang Z, Zhu W, Hu M, Wang H, Chen Z, Shen R, Yu Y, Tan R, Guo S. Secondary Organic Aerosol from Typical Chinese Domestic Cooking Emissions. Environmental Science and Technology LettersEnvironmental Science and Technology LettersEnvironmental Science and Technology Letters. 2021;8:24-31.Abstract
Cooking has been proven to be a significant source of primary organic aerosol, especially in megacities. However, the formation of secondary organic aerosol (SOA) derived from cooking emissions is still poorly understood. In this work, four prevalent Chinese domestic cooking types involving complicated cuisines and various cooking methods were chosen to conduct a lab simulation for SOA formation using a Gothenburg potential aerosol mass reactor (Go: PAM). After samples had been aged under OH exposures of 4.3-27.1 × 1010 molecules cm-3 s, the domestic cooking SOA was characterized by mass growth potentialities (1.81-3.16), elemental ratios (O/C = 0.29-0.41), and mass spectra. Compared with other organic aerosol (OA), domestic cooking SOA is a kind of less oxidized oxygenated OA (LO-OOA) with a unique oxidation pathway (alcohol/peroxide pathway) and mass spectra (characteristic peaks at m/z 28, 29, 41, 43, 44, 55, and 57). This study is expected to identify the cooking SOA under actual cooking conditions, which could contribute to the formulation of pollution source control as well as the health risk assessment of exposure to cooking fumes. ©
Cheng X, Chen Q, Li Y, Huang G, Liu Y, Lu S, Zheng Y, Qiu W, Lu K, Qiu X, et al. Secondary Production of Gaseous Nitrated Phenols in Polluted Urban Environments. Environmental Science & Technology. 2021;55(8):4410-4419.
Cheng X, Chen Q, Li Y, Huang G, Liu Y, Lu S, Zheng Y, Qiu W, Lu K, Qiu X, et al. Secondary Production of Gaseous Nitrated Phenols in Polluted Urban Environments. Environmental Science & Technology [Internet]. 2021:null. 访问链接
Schuller F, Urquhart J  S, Csengeri T, Colombo D, Duarte-Cabral A, Mattern M, Ginsburg A, Pettitt A  R, Wyrowski F, Anderson L, et al. The SEDIGISM survey: First Data Release and overview of the Galactic structure. \mnras. 2021;500:3064-3082.

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