<?xml version="1.0" encoding="UTF-8"?><xml><records><record><source-app name="Biblio" version="7.x">Drupal-Biblio</source-app><ref-type>17</ref-type><contributors><authors><author><style face="normal" font="default" size="100%">Z. Wang</style></author><author><style face="normal" font="default" size="100%">Hu, W.</style></author><author><style face="normal" font="default" size="100%">Niu, H.</style></author><author><style face="normal" font="default" size="100%">Hu, W.</style></author><author><style face="normal" font="default" size="100%">Wu, Y.</style></author><author><style face="normal" font="default" size="100%">L. Wu</style></author><author><style face="normal" font="default" size="100%">Ren, L.</style></author><author><style face="normal" font="default" size="100%">Deng, J.</style></author><author><style face="normal" font="default" size="100%">Guo, S.</style></author><author><style face="normal" font="default" size="100%">Wu, Z.</style></author><author><style face="normal" font="default" size="100%">D. Zhang</style></author><author><style face="normal" font="default" size="100%">Fu, P.</style></author><author><style face="normal" font="default" size="100%">Hu, M.</style></author></authors></contributors><titles><title><style face="normal" font="default" size="100%">Variations in physicochemical properties of airborne particles during a heavy haze-to-dust episode in Beijing</style></title><secondary-title><style face="normal" font="default" size="100%">Science of the Total EnvironmentScience of the Total Environment</style></secondary-title><alt-title><style face="normal" font="default" size="100%">Sci. Total Environ.</style></alt-title><short-title><style face="normal" font="default" size="100%">Sci Total Environ</style></short-title></titles><keywords><keyword><style  face="normal" font="default" size="100%">aerosol formation</style></keyword><keyword><style  face="normal" font="default" size="100%">Aerosol mass spectrometer</style></keyword><keyword><style  face="normal" font="default" size="100%">air pollutant</style></keyword><keyword><style  face="normal" font="default" size="100%">air pollution</style></keyword><keyword><style  face="normal" font="default" size="100%">airborne particle</style></keyword><keyword><style  face="normal" font="default" size="100%">Anthropogenic elements</style></keyword><keyword><style  face="normal" font="default" size="100%">aqueous phase reaction</style></keyword><keyword><style  face="normal" font="default" size="100%">Aqueous phase reactions</style></keyword><keyword><style  face="normal" font="default" size="100%">article</style></keyword><keyword><style  face="normal" font="default" size="100%">atmospheric pollution</style></keyword><keyword><style  face="normal" font="default" size="100%">Beijing [Beijing (ADS)]</style></keyword><keyword><style  face="normal" font="default" size="100%">Beijing [China]</style></keyword><keyword><style  face="normal" font="default" size="100%">black carbon</style></keyword><keyword><style  face="normal" font="default" size="100%">Chemical analysis</style></keyword><keyword><style  face="normal" font="default" size="100%">Chemical composition</style></keyword><keyword><style  face="normal" font="default" size="100%">Chemical compositions</style></keyword><keyword><style  face="normal" font="default" size="100%">chemical reaction</style></keyword><keyword><style  face="normal" font="default" size="100%">China</style></keyword><keyword><style  face="normal" font="default" size="100%">climate</style></keyword><keyword><style  face="normal" font="default" size="100%">coating (procedure)</style></keyword><keyword><style  face="normal" font="default" size="100%">Coatings</style></keyword><keyword><style  face="normal" font="default" size="100%">controlled study</style></keyword><keyword><style  face="normal" font="default" size="100%">dust</style></keyword><keyword><style  face="normal" font="default" size="100%">environment</style></keyword><keyword><style  face="normal" font="default" size="100%">gas</style></keyword><keyword><style  face="normal" font="default" size="100%">haze</style></keyword><keyword><style  face="normal" font="default" size="100%">haze to dust transition</style></keyword><keyword><style  face="normal" font="default" size="100%">Haze-to-dust transition</style></keyword><keyword><style  face="normal" font="default" size="100%">health hazard</style></keyword><keyword><style  face="normal" font="default" size="100%">humidity</style></keyword><keyword><style  face="normal" font="default" size="100%">Individual particles analysis</style></keyword><keyword><style  face="normal" font="default" size="100%">mass spectrometry</style></keyword><keyword><style  face="normal" font="default" size="100%">measurement accuracy</style></keyword><keyword><style  face="normal" font="default" size="100%">mineral</style></keyword><keyword><style  face="normal" font="default" size="100%">On-line measurement</style></keyword><keyword><style  face="normal" font="default" size="100%">ozone</style></keyword><keyword><style  face="normal" font="default" size="100%">Particle size</style></keyword><keyword><style  face="normal" font="default" size="100%">Particle size analysis</style></keyword><keyword><style  face="normal" font="default" size="100%">particulate matter</style></keyword><keyword><style  face="normal" font="default" size="100%">particulate matter 10</style></keyword><keyword><style  face="normal" font="default" size="100%">photochemical oxidation</style></keyword><keyword><style  face="normal" font="default" size="100%">photooxidation</style></keyword><keyword><style  face="normal" font="default" size="100%">physical chemistry</style></keyword><keyword><style  face="normal" font="default" size="100%">Physicochemical properties</style></keyword><keyword><style  face="normal" font="default" size="100%">physicochemical property</style></keyword><keyword><style  face="normal" font="default" size="100%">priority journal</style></keyword><keyword><style  face="normal" font="default" size="100%">scanning electron microscopy</style></keyword><keyword><style  face="normal" font="default" size="100%">secondary formation</style></keyword><keyword><style  face="normal" font="default" size="100%">secondary particles</style></keyword><keyword><style  face="normal" font="default" size="100%">Single-particle analysis</style></keyword><keyword><style  face="normal" font="default" size="100%">soot</style></keyword><keyword><style  face="normal" font="default" size="100%">Sub-micron particles</style></keyword><keyword><style  face="normal" font="default" size="100%">sulfur</style></keyword><keyword><style  face="normal" font="default" size="100%">surface property</style></keyword><keyword><style  face="normal" font="default" size="100%">weather</style></keyword></keywords><dates><year><style  face="normal" font="default" size="100%">2021</style></year></dates><volume><style face="normal" font="default" size="100%">762</style></volume><language><style face="normal" font="default" size="100%">eng</style></language><abstract><style face="normal" font="default" size="100%">The variations in physicochemical properties of airborne particles collected during a typical transition from haze to dust were investigated using single particle analysis with transmission and scanning electron microscopes combined with online measurement of chemical compositions of airborne particles in Beijing in February 2013. The transition was divided into three phases based on the weather condition. During haze pollution (Phase 1), gaseous and particle pollutants enhanced gradually. Results from single particle analysis showed that more coatings and more anthropogenic elements (e.g., S) appeared on the surface of fine and coarse particles, which was probably caused by efficient aqueous-phase reactions under high humidity (70%) condition. Phase 2 was dust intrusion episode. PM10 reached over 1000 μg m−3. Larger fractions of mineral particles and bare-like soot particles were observed in fine particles, while the fraction of secondary particles with coatings decreased. The proportion of black carbon in submicron particles also increased. Photochemical oxidation in gas phase likely dominated in secondary formation under high O3 concentration. After the dust episode (Phase 3), secondary formation enhanced obviously. Soot aged quickly and had a larger mode of 0.45 μm than the other phases. The size modes of airborne fine particles during Phases 1 and 3 were 0.35 μm, which were a bit larger than that during Phase 2 (0.24 μm). These results indicate that dust plumes accompanied with strong wind brought mineral particles in both fine and coarse modes and freshly emitted particles with smaller sizes, and swept away pre-presence air pollutants. This study could provide detailed information on the physicochemical properties of airborne particles during typical severe pollution processes in a short time. Such short-term change should be taken into account in order to more accurately assess the environmental, climatic and health-related effects of airborne particles. © 2020 Elsevier B.V.</style></abstract><work-type><style face="normal" font="default" size="100%">Article</style></work-type><notes><style face="normal" font="default" size="100%">施引文献 :1Export Date: 7 June 2021</style></notes><custom7><style face="normal" font="default" size="100%">143081</style></custom7><remote-database-name><style face="normal" font="default" size="100%">Scopus</style></remote-database-name></record></records></xml>