科研成果

2018
Gao X, Zhang Y, Schottker B, Brenner H. Vitamin D status and epigenetic-based mortality risk score: strong independent and joint prediction of all-cause mortality in a population-based cohort study. Clin Epigenetics [Internet]. 2018;10:84. 访问链接Abstract
Background: Vitamin D deficiency and insufficiency have been established to be strongly associated with increased overall mortality and deaths from specific aging-related diseases. Recently, an epigenetic "mortality risk score" (MS) based on whole blood DNA methylation at the 10 most prominent mortality-related cytosine-phosphate-guanine (CpG) sites has also been found to be highly related to all-cause mortality. This study aimed to explore whether vitamin D status, defined by serum 25-hydroxyvitamin D [25(OH)D] concentrations, is associated with the MS and to what extent both indicators are individually and jointly capable of predicting all-cause mortality in a general population sample of older adults. Results: The MS was derived from the blood DNA methylation profiles measured by Illumina Human Methylation 450K Beadchip, and serum 25(OH)D concentration was measured among 1467 participants aged 50-75 of the German ESTHER cohort study. There was no association between vitamin D status and the MS at baseline, but both metrics were prominently and independently associated with all-cause mortality during a median follow-up of 15.2 years. The combination of both indicators showed the potential to be a particularly strong prognostic index for all-cause mortality. Participants with vitamin D deficiency (< 30 nmol/L) and high MS (> 5 CpG sites with aberrant methylation) had almost sixfold mortality (hazard ratio 5.79, 95% CI 3.06-10.94) compared with participants with sufficient vitamin D (>/= 50 nmol/L) and a low MS (0-1 CpG site with aberrant methylation). Conclusions: This study suggests that vitamin D and the MS are strong independent predictors of all-cause mortality in older adults.
Zhang H, Liu Y, Yang C, Xiang L, Hu Y*, Peng L-M*. Wafer-Scale Fabrication of Ultrathin Flexible Electronic Systems via Capillary-Assisted Electrochemical Delamination. Advanced Materials. 2018;30:1805408.
Zhang H, Liu Y, Yang C, Xiang L, Hu Y*, Peng L-M*. Wafer-Scale Fabrication of Ultrathin Flexible Electronic Systems via Capillary-Assisted Electrochemical Delamination. Advanced Materials. 2018;30:1805408.
Zhang H, Liu Y, Yang C, Xiang L, Hu Y*, Peng L-M*. Wafer-Scale Fabrication of Ultrathin Flexible Electronic Systems via Capillary-Assisted Electrochemical Delamination. Advanced Materials. 2018:1805408.
Zhang H, Liu Y, Yang C, Xiang L, Hu Y*, Peng L-M*. Wafer-Scale Fabrication of Ultrathin Flexible Electronic Systems via Capillary-Assisted Electrochemical Delamination. Advanced Materials. 2018:1805408.
Song QY, Meng XR, Hinney A, Song JY, Huang T, Ma J, Wang HJ. Waist-hip ratio related genetic loci are associated with risk of impaired fasting glucose in Chinese children: a case control study. Nutr Metab (Lond)Nutr Metab (Lond)Nutr Metab (Lond). 2018;15:34.Abstract
Background: The meta-analyses of genome-wide association studies identified several waist-hip ratio (WHR) related loci in individuals of European ancestry. Since the pattern of fat distribution and the relationship between fat distribution and glucose metabolism disturbance in Chinese are different from those in Europeans, the present study aimed to explore the individual and cumulative effects of WHR-related loci on glycemic phenotypes in Chinese children. Methods: A total of 2030 children were recruited from two independent studies. Eleven single nucleotide polymorphisms (SNPs) were selected and genotyped using matrix-assisted laser desorption ionization time of flight mass spectrometry (MALDI-TOF MS). Logistic regression and linear regression model were used to examine the association of 11 SNPs and genetic risk score (GRS) with impaired fasting glucose (IFG) and fasting plasma glucose (FPG), respectively. Results: Three SNPs (rs6795735, rs984222 and rs1011731) were nominally associated with IFG (all P < 0.05). Each WHR-increasing (C) allele of rs6795735 (ADAMTS9) was associated with a 40.1% increased risk of IFG (OR = 1.401, 95% CI = 1.131-1.735, P = 0.002), which remained significant after Bonferroni correction. We observed no association of both weighted and unweighted GRS with FPG and IFG (all P > 0.05). Conclusions: We identified individual effects of rs6795735 (ADAMTS9), rs984222 (TBX15-WARS2), and rs1011731 (DNM3-PIGC) on glycemic phenotypes in Chinese children for the first time. The study suggests that genetic predisposition to central obesity is associated with impaired fasting glucose, providing more evidence for the pathogenesis of diabetes.
Wang Q.L., Wei W., Liu S.T., Yan M.Q., Song K., Mai J., et al., 2018. Free ammonia pretreatment improves degradation of secondary sludge during aerobic digestion. ACS Sustainable Chemistry & Engineering 6(1),1105-1111. 2018.
Chen X, Miao L, Guo H, Chen H, Song Y, Su Z, Zhang H. Waterproof and stretchable triboelectric nanogenerator for biomechanical energy harvesting and self-powered sensing. Applied Physics Letters. 2018;112(20):203902.
Yu H, Cheng X, Wang Y, Liu Y, Rong K, Li Z, Wan Y, Gong W, Watanabe K, Taniguchi T, et al. Waterproof perovskite-hexagonal boron nitride hybrid nanolasers with low lasing thresholds and high operating temperature. ACS Photonics [Internet]. 2018;5:4520-4528. 访问链接
Song Y, Song Z, Chen H, Chen X, Guo H, Wu H, Cheng XL, Zhang H. Wearable stretchable double-sided micro-supercapacitors with porous conductive elastomers. Micro Electro Mechanical Systems (MEMS), 2018 IEEE. 2018:608-611.
Cheng XL, Song Z, Miao L, Guo H, Su Z, Song Y, Zhang H-X. Wide Range Fabrication of Wrinkle Patterns for Maximizing Surface Charge Density of a Triboelectric Nanogenerator. Journal of Microelectromechanical Systems. 2018;27(1):106-112.
Du W, Chen Y, Shen G, Wang W, Zhuo S, Huang Y, Pan X, Tao S. Winter air pollution by and inhalation exposure to nitrated and oxygenated PAHs in rural Shanxi, north China. Atmospheric Environment [Internet]. 2018;187:210-217. 访问链接
Du W, Chen Y, Zhu X, Zhong Q, Zhuo S, Liu W, Huang Y, Shen G, Tao S. Wintertime air pollution and health risk assessment of inhalation exposure to polycyclic aromatic hydrocarbons in rural China. Atmospheric Environment [Internet]. 2018;191:1-8. 访问链接
Tan Z, Rohrer F, Lu K, Ma X, Bohn B, Broch S, Dong HB, Fuchs H, Gkatzelis GI, Hofzumahaus A, et al. Wintertime photochemistry in Beijing: observations of ROx radical concentrations in the North China Plain during the BEST-ONE campaign. Atmospheric Chemistry and Physics. 2018;18(16):12391–12411.Abstract
The first wintertime in situ measurements of hydroxyl (OH), hydroperoxy (HO2) and organic peroxy (RO2) radicals (ROx = OH + HO2 + RO2) in combination with observations of total reactivity of OH radicals, k(OH) in Beijing are presented. The field campaign "Beijing winter finE particle STudy - Oxidation, Nucleation and light Extinctions" (BEST-ONE) was conducted at the suburban site Huairou near Beijing from January to March 2016. It aimed to understand oxidative capacity during wintertime and to elucidate the secondary pollutants' formation mechanism in the North China Plain (NCP). OH radical concentrations at noontime ranged from 2.4 x 10(6) cm(-3) in severely polluted air (k(OH) similar to 27s 1 / to 3.6 x 10(6) cm(-3) in relatively clean air (k(OH) similar to 5 s(-1)). These values are nearly 2-fold larger than OH concentrations observed in previous winter campaigns in Birmingham, Tokyo, and New York City. During this campaign, the total primary production rate of ROx radicals was dominated by the photolysis of nitrous acid accounting for 46% of the identified primary production pathways for ROx radicals. Other important radical sources were alkene ozonolysis (28 %) and photolysis of oxygenated organic compounds (24 %). A box model was used to simulate the OH, HO2 and RO2 concentrations based on the observations of their long-lived precursors. The model was capable of reproducing the observed diurnal variation of the OH and peroxy radicals during clean days with a factor of 1.5. However, it largely un-derestimated HO2 and RO2 concentrations by factors up to 5 during pollution episodes. The HO2 and RO2 observed-to-modeled ratios increased with increasing NO concentrations, indicating a deficit in our understanding of the gas-phase chemistry in the high NOx regime. The OH concentrations observed in the presence of large OH reactivities indicate that atmospheric trace gas oxidation by photochemical processes can be highly effective even during wintertime, thereby facilitating the vigorous formation of secondary pollutants.
Tan ZF, Rohrer F, Lu KD, Ma XF, Bohn B, Broch S, Dong HB, Fuchs H, Gkatzelis G, Hofzumahaus A, et al. Wintertime photochemistry in Beijing: Observations of ROx radical concentrations in the North China Plain during the BEST-ONE campaign. Atmos. Chem. Phys. [Internet]. 2018. 访问链接Abstract
The first wintertime in-situ measurements of hydroxyl (OH), hydroperoxy (HO2) and organic peroxy (RO2) radicals (ROx=OH+HO2+RO2) in combination with observations of total reactivity of OH radicals, kOH in Beijing are presented. The field campaign “Beijing winter finE particle STudy – Oxidation, Nucleation and light Extinctions” (BEST-ONE) was conducted at the suburban site Huairou near Beijing from January to March 2016. It aimed to understand oxidative capacity during wintertime and to elucidate the secondary pollutants formation mechanism in the North China Plain (NCP). OH radical concentrations at noontime ranged from 2.4×106cm−3 in severely polluted air (kOH~27s−1) to 3.6×106cm−3 in relatively clean air (kOH~5s−1). These values are nearly two-fold larger than OH concentrations observed in previous winter campaign in Birmingham, Tokyo, and New York City. During this campaign, the total primary production rate of ROx radicals was dominated by the photolysis of nitrous acid accounting for 46% of the identified primary production pathways for ROxradicals. Other important radical sources were alkene ozonolysis (28%) and photolysis of oxygenated organic compounds (24%). A box model was used to simulate the OH, HO2 and RO2 concentrations based on the observations of their long-lived precursors. The model was capable of reproducing the observed diurnal variation of the OH and peroxy radicals during clean days with a factor of 1.5. However, it largely underestimated HO2 and RO2 concentrations by factors up to 5 during pollution episodes. The HO2 and RO2 observed-to-modeled ratios increased with increasing NO concentrations, indicating a deficit in our understanding of the gas-phase chemistry in the high NOxregime. The OH concentrations observed in the presence of large OH reactivities indicate that atmospheric trace gas oxidation by photochemical processes can be highly effective even during wintertime, thereby facilitating the vigorous formation of secondary pollutants.
Brdar V, Kopp J, Liu J, Wang X-P. X-Ray Lines from Dark Matter Annihilation at the keV Scale. Phys. Rev. Lett. 2018;120:061301.
Yan M.Q.*, Chen Z.H., Li N., Zhou Y.X., Zhang C.Y., Korshin G. 2018. Electrochemical reductive dehalogenation of iodine-containing contrast agent pharmaceuticals: Examination of reactions of diatrizoate and iopamidol using the method of rotating ring-disc. 2018.
Zhang C.Y., Li M.Y., Han X.Z., Yan M.Q.* 2018. Quantum chemical examination of the sequential halogen incorporation scheme for the modeling of speciation of I/Br/Cl-containing trihalomethanes. Environ Sci Technol 52(4), 2162-2169. 2018.
Wang D, Wu C, Luo W, Guo X, Qu B, Xiao L, Chen Z. ZnO/SnO2 Double Electron Transport Layer Guides Improved Open Circuit Voltage for Highly Efficient CH3NH3PbI3-Based Planar Perovskite Solar Cells. ACS APPLIED ENERGY MATERIALS. 2018;1:2215-2221.
贺勇, 师晓敏, 张敏, 史俊杰. ZnO1-xRx (R=S, Se, Te) 电子结构与光学性质的第一性原理研究. 内蒙古大学学报. 自然科学版 [Internet]. 2018;49(3):270-278. 访问链接

Pages