科研成果

2020
Xie Y, Liu XR, Chen Q, Zhang SH. An integrated assessment for achieving the 2 degrees C target pathway in China by 2030. Journal of Cleaner Production. 2020;268.Abstract
China submitted the Greenhouse gas emission reduction target in the form of Nationally Determined Contributions (NDC) to the Paris Agreement. To reduce the negative impact of global warming, a tighter target is needed, such as the 2-degree target. This study investigated how China could reach its emissions peak and decarbonize its economy through different key countermeasures in various sectors in line with the NDC and 2 degrees C targets by 2030. A dynamic CGE model is used to develop ten scenarios that contain two dimensions consisting of two stringency levels of carbon emission limitation and the availability of different low-carbon options. We found that in the baseline scenario, China's total CO2 emissions in 2030 would reach 14.7 Gt. To meet China's NDC target, it is essential to develop non-fossil fuel energy, restrict the over-expansion of energy-intensive industries and improve end-use efficiency. Meanwhile, the global 2 degrees C target poses higher requirements for China to develop various non-fossil technologies both in electricity production and demand sectors, and vigorously promote low-carbon consumption pattern. Furthermore, we estimated the economic impacts and found that if low-carbon measures are adopted properly, the mitigation cost in 2030 could decline by 92 and 226 USD/ton-CO2 under the NDC target and 2 degrees C target, respectively. Accordingly, GDP loss could fall from 3.8% to barely 0.004% under the NDC target, and from 11.6% to 1.6% under the 2 degrees C target. The welfare will almost not be affected significantly under all scenarios. Moreover, carbon reduction will also bring co-benefits on the air pollution improvement in China. (c) 2020 Elsevier Ltd. All rights reserved.
Guo J-X, Huang C, Wang J-L, Meng X-Y. Integrated operation for the planning of CO2 capture path in CCS–EOR project. Journal of Petroleum Science and Engineering. 2020;186.Abstract
© 2019 Elsevier B.V. Carbon utilization and storage (CCUS) project represented by enhanced oil recovery (EOR) technology provides a feasible way for the CCS dynamic cost to decline. With the development of CCS and the cost reduction of power plant capture, the possibility of oil companies receiving CO2 from power plants will increase, which makes CO2 and oil resources more fully utilized. Based on this fact, this work proposes a novel model regarding the CCS–EOR project to systematically evaluate the CCS development path and the EOR utilization process. By considering the CO2 source captured by CCS and the utilization process of EOR process, the cost-benefit model of integrated system is established, and the CO2 capture/injection path of CCS/EOR is optimized. This model helps to analyze CCS investment and carbon capture process from the perspective of the whole project process, and provides a feasible reference for practical large-scale engineering decision-making project.
Kim D, Yamauchi Y, Meng X, Jia T, McAuliffe L, Takken T, Tien K, Tian S, Yao Y, Ferencz A, et al. An integrated programmable gate timing control and gate driver chip for a 48V-to-0.75V active-clamp forward converter power block, in Energy Conversion Congress and Exposition (ECCE).; 2020.
Cheng Z, Wheeler VD, Bai T, Shi J, Tadjer MJ, Feygelson T, Hobart KD, Goorsky MS, Graham S. Integration of polycrystalline Ga2O3 on diamond for thermal management. Applied Physics Letters. 2020;116(6):062105.
Cheng Z, Wheeler VD, Bai T, Shi J, Tadjer MJ, Feygelson T, Hobart KD, Goorsky MS, Graham S. Integration of polycrystalline Ga2O3 on diamond for thermal management. Applied Physics Letters. 2020;116(6):062105.
Yang Z, Sun H, Wu W. Intensified simultaneous nitrification and denitrification performance in integrated packed bed bioreactors using PHBV with different dosing methods. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH. 2020;27:21560-21569.Abstract
To explore an effective approach of simultaneous nitrification and denitrification in wastewater with low C/N ratios, integrated packed bed bioreactors based on poly(3-hydroxybutyrate-hydroxyvalerate) (PHBV) with different dosing methods were designed. The removal efficiency of NH4+-N in bioreactor with aeration was 88.62%, and higher NO3–N removal efficiency was observed in bioreactor filled with grainy PHBV (95.21%) than bioreactor filled with strip PHBV (93.34%). Microbial study indicated that microbes harboring amoA and nirS genes preferred to attach on the surface of ceramsite, and significant differences in microbial community compositions at phylum and genus levels were observed. To summarize, it is feasible to utilize grainy PHBV for simultaneous and efficient removal of NH4+-N and NO3–N from wastewater with low C/N ratios.
Cheng Z, Mu F, Yates L, Suga T, Graham S. Interfacial Thermal Conductance across Room-Temperature-Bonded GaN/Diamond Interfaces for GaN-on-Diamond Devices. ACS Applied Materials & Interfaces. 2020;12(7):8376-8384.
Fang Z, Li X, Shi W, Li Z, Guo Y, Chen Q, Peng LM, Wei X. Interlayer Binding Energy of Hexagonal MoS2 as Determined by an In Situ Peeling-to-Fracture Method. The Journal of Physical Chemistry C [Internet]. 2020;124:23419-23425. 访问链接
Kalesan B, Zhao S, Poulson M, Neufeld M, Dechert T, Siracuse JJ, Zuo Y, Li F. Intersections of Firearm Suicide, Drug-Related Mortality, and Economic Dependency in Rural America. Journal of Surgical Research. 2020;256:96–102.
An L*, Tang Y, Wang D, Jia S, Pei Q, Wang Q, Yu Z*, Liu JK. Intrinsic and Synaptic Properties Shaping Diverse Behaviors of Neural Dynamics. Frontiers in Computational Neuroscience [Internet]. 2020;14:26. PDFAbstract
The majority of neurons in the neuronal systems of the brain have a complex structure of the morphology, which diversifies the dynamics of neurons. In the granule layer of the cerebellum, there exists a unique cell type, unipolar brush cell (UBC), serving as an important relay cell to transfer information from outside mossy fibers to downstream granule cells. The distinguishing feature of UBC is that it has a simple morphology with only one short dendritic brush connected its soma. Based on experimental evidence showing that UBCs exhibit a variety of dynamic behaviors, here we develop two simple models, one with a few detailed ion channels for simulation, and the other one as a two-variable dynamical system for theoretical analysis, to characterize the intrinsic dynamics of UBCs. The reasonable values of the key channel parameters of the models can be determined by analysis of the stability of the resting membrane potential and the rebound firing properties of UBCs. Together with a large variety of synaptic dynamics installed on UBCs, we show the simple structured UBCs, as relay cells, can extend the range of dynamics and information from input mossy fibers to granular cells with low-frequency resonance, and transfer the stereotyped input to diverse amplitudes and phases of the output for downstream granule cells. These results suggest that neuronal computation, embedded with intrinsic ion channels and diverse synaptic properties on single neurons without sophisticated morphology, can shape a large variety of dynamic behaviors to enhance the computational ability of local neuronal circuits.
Garay MJ, Witek ML, Kahn RA, Seidel FC, Limbacher JA, Bull MA, Diner DJ, Hansen EG, Kalashnikova OV, Lee H, et al. Introducing the 4.4 km spatial resolution Multi-Angle Imaging SpectroRadiometer (MISR) aerosol product. Atmospheric Measurement Techniques. 2020;13:593–628.
Investigation of electron vortices in time-delayed circularly polarized laser pulses with a semiclassical perspective. Optics Express [Internet]. 2020;28(20): 29442-29454. 访问链接Abstract
We theoretically investigate strong-filed electron vortices in time-delayed circularly polarized laser pulses by a generalized quantum-trajectory Monte Carlo (GQTMC) model. Vortex interference patterns in photoelectron momentum distributions (PMDs) with various laser parameters can be well reproduced by the semiclassical simulation. The phase difference responsible for the interference structures is analytically identified through trajectory-based analysis and simple-man theory, which reveal the underlying mechanism of electron vortex phenomena for both co-rotating and counter-rotating component. This semiclassical analysis can also demonstrate the influences of laser intensity and wavelength on the number of arms of vortices. Furthermore, we show the influence of the Coulomb effect on the PMDs. Finally, the controlling of the ionization time intervals in the tens to hundreds of attosecond magnitude is qualitatively discussed.
Zhao Z, Bu Y, Kang L, Min C, Bian Y, Tang L, Li J. An investigation of the relationship between scientists’ mobility to/from China and their research performance. Journal of Informetrics. 2020;14(2):101037.
Shi X, Qiu X, Cheng Z, Chen Q, Rudich Y, Zhu T. Isomeric identification of particle-phase organic nitrates through gas chromatography and time-of-flight mass spectrometry coupled with an electron capture negative ionization source. Environmental Science & Technology. 2020;54:707-713.
Sheng A, Liu J, Li X, Qafoku O, Collins RN, Jones AM, Pearce CI, Wang C, Ni J, Lu A, et al. Labile Fe(III) from sorbed Fe(II) oxidation is the key intermediate in Fe(II)-catalyzed ferrihydrite transformation. Geochimica et Cosmochimica Acta [Internet]. 2020;272:105 - 120. 访问链接Abstract
Ferrihydrite (Fh) is a major Fe(III)-(oxyhydr)oxide nanomineral distinguished by its poor crystallinity and thermodynamic metastability. While it is well known that in suboxic conditions aqueous Fe(II) rapidly catalyzes Fh transformation to more stable crystalline Fe(III) phases such as lepidocrocite (Lp) and goethite (Gt), because of the low solubility of Fe(III) the mass transfer pathways enabling these rapid transformations have remained unclear for decades. Here, using a selective extractant, we isolated and quantified a critical labile Fe(III) species, one that is more reactive than Fe(III) in Fh, formed by the oxidation of aqueous Fe(II) on the Fh surface. Experiments that compared time-dependent concentrations of solid-associated Fe(II) and this labile Fe(III) against the kinetics of phase transformation showed that its accumulation is directly related to Lp/Gt formation in a manner consistent with the classical nucleation theory. 57Fe isotope tracer experiments confirm the oxidized Fe(II) origin of labile Fe(III). The transformation pathway as well as the accelerating effect of Fe(II) can now all be explained on a unified basis of the kinetics of Fe(III) olation and oxolation reactions necessary to nucleate and sustain growth of Lp/Gt products, rates of which are greatly accelerated by labile Fe(III).
Alam MK, Niu C, Wang Y, Wang W, Li Y, Dai C, Tong T, Shan X, Charlson E, Pei S, et al. Large graphene-induced shift of surface-plasmon resonances of gold films: Effective-medium theory for atomically thin materials. Physical Review Research [Internet]. 2020;2:013008. LinkAbstract
espite successful modeling of graphene as a 0.34-nm-thick optical film synthesized by exfoliation or chemical vapor deposition (CVD), graphene-induced shift of surface-plasmon resonance (SPR) of gold films has remained controversial. Here we report the resolution of this controversy by developing a clean CVD graphene transfer method and extending Maxwell-Garnett effective-medium theory (EMT) to two-dimensional (2D) materials. A SPR shift of 0.24° is obtained and it agrees well with 2D EMT in which wrinkled graphene is treated as a 3-nm graphene/air layered composite, in agreement with the average roughness measured by atomic force microscopy. Because the anisotropic built-in boundary condition of 2D EMT is compatible with graphene's optical anisotropy, graphene can be modeled as a film thicker than 0.34 nm without changing its optical property; however, its actual roughness, i.e., effective thickness, will significantly alter its response to strong out-of-plane fields, leading to a larger SPR shift.
b a a a b Jie Wang a, ⁎ MHQWYSYZYH. LDPE microplastics significantly alter the temporal turnover of soil microbial communities. Science of the Total Environment [Internet]. 2020;726:138682-. 访问链接
Li Y, Reich PB, Schmid B, Shrestha N, Feng X, Lyu T, Maitner BS, Xu X, Li Y, Zou D, et al. Leaf size of woody dicots predicts ecosystem primary productivity. Ecology LettersEcology LettersEcology Letters. 2020;23:1003-1013.Abstract
Abstract A key challenge in ecology is to understand the relationships between organismal traits and ecosystem processes. Here, with a novel dataset of leaf length and width for 10 480 woody dicots in China and 2374 in North America, we show that the variation in community mean leaf size is highly correlated with the variation in climate and ecosystem primary productivity, independent of plant life form. These relationships likely reflect how natural selection modifies leaf size across varying climates in conjunction with how climate influences canopy total leaf area. We find that the leaf size‒primary productivity functions based on the Chinese dataset can predict productivity in North America and vice-versa. In addition to advancing understanding of the relationship between a climate-driven trait and ecosystem functioning, our findings suggest that leaf size can also be a promising tool in palaeoecology for scaling from fossil leaves to palaeo-primary productivity of woody ecosystems.
Yang L, Wu H, Zhang T, Cheng X, Li F, Zou L, Wang Y, Chen R, Wang J, Huang G. Leaper: A Learned Prefetcher for Cache Invalidation in LSM-tree based Storage Engines. Proc. VLDB Endow. 2020;13:1976–1989.
Zhou Y, Guo J, Wang Z, Zhang B, Sun Z, Yun X, Zhang J. Levels and inhalation health risk of neonicotinoid insecticides in fine particulate matter (PM2.5) in urban and rural areas of China. Environment International [Internet]. 2020;142. 访问链接Abstract
Neonicotinoid insecticide (NEO) concentrations in ambient fine particulate matter (PM2.5) and daily exposure via inhalation were investigated during spring and fall in an urban area in Beijing and in urban and rural areas of Zhengzhou, Henan Province, China. Four NEOs, including imidacloprid, acetamiprid, thiamethoxam and clothianidin, were assessed using a QuEChERS (quick, easy, cheap, effective, rugged, safe) extraction procedure coupled to liquid chromatography–tandem mass spectrometry. Of 64 PM2.5 samples, 100% contained at least two NEOs (imidacloprid and acetamiprid). Imidacloprid was detected at the highest levels, ranging from 4.33 to 1.13 × 102 pg m−3. A relative potency factor method that considered different toxicities was used to integrate the four NEO concentrations. The total NEO concentrations in air in the Zhengzhou rural area (mean: 80.86 pg m−3) were higher than those in urban areas. Differences between seasons were not significant (p > 0.05). The highest value for the total average daily dose via inhalation of four NEOs (ADDinh,total), 91.0 pg kg−1 day−1, was found in rural children <6 years old. The ADDinh,total of rural residents was significantly higher than that of urban residents when there was no intensive pesticide application. Although the ADDinh,total values were below the current chronic reference dose, when possible joint toxicity and the increasing use of NEOs are considered, a potential health risk via inhalation is evident. We believe this study is the first to characterize NEO levels in fine particulate matter and to evaluate inhalation exposure in urban and rural residents under nonoccupational scenarios in China. It will enhance our understanding of exposure to NEOs and provide a basis for risk management decisions. © 2020 The Author(s)

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